Electrically Accessible Metamagnetic Transition via a Doping-Induced Low-Energy Magnetic State in Antiferromagnetic Insulator RFeO3

Fuente: arXiv
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Autori principali: Yang, Wanting, Peng, Haohuan, Wang, Ziming, Ma, Xiaoxuan, Kang, Baojuan, Xue, Chang, Jia, Rongrong, Ge, Jun-Yi, Cheng, Jinrong, Cao, Shixun
Natura: Preprint
Pubblicazione: 2026
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author Yang, Wanting
Peng, Haohuan
Wang, Ziming
Ma, Xiaoxuan
Kang, Baojuan
Xue, Chang
Jia, Rongrong
Ge, Jun-Yi
Cheng, Jinrong
Cao, Shixun
author_facet Yang, Wanting
Peng, Haohuan
Wang, Ziming
Ma, Xiaoxuan
Kang, Baojuan
Xue, Chang
Jia, Rongrong
Ge, Jun-Yi
Cheng, Jinrong
Cao, Shixun
contents Low-energy antiferromagnetic phase transitions offer an appealing platform for low-power spintronic functionalities, yet their direct electrical access in insulating antiferromagnets remains challenging, particularly in the low-field regime where subtle Neeel vector reorientations dominate. Here, we demonstrate that targeted rare-earth-site engineering enables an electrically accessible metamagnetic transition in the insulating orthoferrite Ho0.5Dy0.5FeO3. By combining the distinct spin-reorientation sequences of DyFeO3 and HoFeO3, Dy substitution stabilizes a dual spin-reorientation pathway, hosting an intermediate state with a reduced energy barrier. This low-energy antiferromagnetic state can be tuned into the weak-ferromagnetic state under low magnetic fields. The critical field decreases with increasing temperature, providing a favorable window for functional manipulation. Both longitudinal and transverse spin Hall magnetoresistance channels exhibit clear and reproducible signatures of the metamagnetic transitions. Owing to the enhanced sensitivity of the transverse channel, additional low-field features are resolved, reflecting the projection of the Neel vector onto the spin-accumulation direction. Electrical transport measurements correlate directly with the magnetically determined phase boundaries, establishing a purely electrical access to low-energy phase transitions and to illustrate a viable pathway for exploring low-power spin dynamics in insulating oxide antiferromagnets.
format Preprint
id arxiv_https___arxiv_org_abs_2601_16501
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Electrically Accessible Metamagnetic Transition via a Doping-Induced Low-Energy Magnetic State in Antiferromagnetic Insulator RFeO3
Yang, Wanting
Peng, Haohuan
Wang, Ziming
Ma, Xiaoxuan
Kang, Baojuan
Xue, Chang
Jia, Rongrong
Ge, Jun-Yi
Cheng, Jinrong
Cao, Shixun
Materials Science
Low-energy antiferromagnetic phase transitions offer an appealing platform for low-power spintronic functionalities, yet their direct electrical access in insulating antiferromagnets remains challenging, particularly in the low-field regime where subtle Neeel vector reorientations dominate. Here, we demonstrate that targeted rare-earth-site engineering enables an electrically accessible metamagnetic transition in the insulating orthoferrite Ho0.5Dy0.5FeO3. By combining the distinct spin-reorientation sequences of DyFeO3 and HoFeO3, Dy substitution stabilizes a dual spin-reorientation pathway, hosting an intermediate state with a reduced energy barrier. This low-energy antiferromagnetic state can be tuned into the weak-ferromagnetic state under low magnetic fields. The critical field decreases with increasing temperature, providing a favorable window for functional manipulation. Both longitudinal and transverse spin Hall magnetoresistance channels exhibit clear and reproducible signatures of the metamagnetic transitions. Owing to the enhanced sensitivity of the transverse channel, additional low-field features are resolved, reflecting the projection of the Neel vector onto the spin-accumulation direction. Electrical transport measurements correlate directly with the magnetically determined phase boundaries, establishing a purely electrical access to low-energy phase transitions and to illustrate a viable pathway for exploring low-power spin dynamics in insulating oxide antiferromagnets.
title Electrically Accessible Metamagnetic Transition via a Doping-Induced Low-Energy Magnetic State in Antiferromagnetic Insulator RFeO3
topic Materials Science
url https://arxiv.org/abs/2601.16501