Shake-up and shake-off spectra in the electron capture decay of atomic $^7$Be

Fuente: arXiv
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Autori principali: Guerra, Mauro, Kim, Inwook, Friedrich, Stephan, Amaro, Pedro, Andoche, Adrien, Baptista, Gonçalo, Bray, Connor, Cantor, Robin, Diercks, David, Fretwell, Spencer L., Gillespie, Abigail, Hall, Ad, Harris, Cameron N., Harris, Jackson T., Hayen, Leendert M., Hervieux, Paul Antoine, Indelicato, Paul, Kim, Geon Bo, Leach, Kyle G., Lennarz, Annika, Lordi, Vincenzo, Machule, Peter, Marino, Andrew, McKeen, David, Mougeot, Xavier, Pinheiro, Daniel, Ponce, Francisco, Ruiz, Chris, Samanta, Amit, Santos, José Paulo, Smolsky, Joseph, Stone-Whitehead, Caitlyn, Templet, Joseph, Warburton, William K., Waters, Benjamin, Machado, Jorge
Natura: Preprint
Pubblicazione: 2026
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author Guerra, Mauro
Kim, Inwook
Friedrich, Stephan
Amaro, Pedro
Andoche, Adrien
Baptista, Gonçalo
Bray, Connor
Cantor, Robin
Diercks, David
Fretwell, Spencer L.
Gillespie, Abigail
Hall, Ad
Harris, Cameron N.
Harris, Jackson T.
Hayen, Leendert M.
Hervieux, Paul Antoine
Indelicato, Paul
Kim, Geon Bo
Leach, Kyle G.
Lennarz, Annika
Lordi, Vincenzo
Machule, Peter
Marino, Andrew
McKeen, David
Mougeot, Xavier
Pinheiro, Daniel
Ponce, Francisco
Ruiz, Chris
Samanta, Amit
Santos, José Paulo
Smolsky, Joseph
Stone-Whitehead, Caitlyn
Templet, Joseph
Warburton, William K.
Waters, Benjamin
Machado, Jorge
author_facet Guerra, Mauro
Kim, Inwook
Friedrich, Stephan
Amaro, Pedro
Andoche, Adrien
Baptista, Gonçalo
Bray, Connor
Cantor, Robin
Diercks, David
Fretwell, Spencer L.
Gillespie, Abigail
Hall, Ad
Harris, Cameron N.
Harris, Jackson T.
Hayen, Leendert M.
Hervieux, Paul Antoine
Indelicato, Paul
Kim, Geon Bo
Leach, Kyle G.
Lennarz, Annika
Lordi, Vincenzo
Machule, Peter
Marino, Andrew
McKeen, David
Mougeot, Xavier
Pinheiro, Daniel
Ponce, Francisco
Ruiz, Chris
Samanta, Amit
Santos, José Paulo
Smolsky, Joseph
Stone-Whitehead, Caitlyn
Templet, Joseph
Warburton, William K.
Waters, Benjamin
Machado, Jorge
contents The most stringent laboratory-based experimental limits on the existence of sub-MeV sterile neutrinos are currently set by decay spectroscopy of radioactive $^7$Be embedded into superconducting sensors. The systematic uncertainties are dominated by the modeling of the electron shake-up and shake-off spectra that are not based on state-of-the-art atomic theory and do not include electron correlations or relativistic effects. We have used the multiconfiguration Dirac-Fock formalism to obtain correlated wavefunctions ab initio and compute all single and double shake processes in the electron capture decay of atomic $^7$Be. The simulations can explain some but not all of the observed spectral features, likely because the wave functions are modified by the Ta sensor material that the $^7$Be is embedded into. The new models also show that the L/K electron capture ratio of $^7$Be in Ta has previously been slightly underestimated revising the previous value of 0.070(7) to a new value of 0.0756(20).
format Preprint
id arxiv_https___arxiv_org_abs_2601_16756
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Shake-up and shake-off spectra in the electron capture decay of atomic $^7$Be
Guerra, Mauro
Kim, Inwook
Friedrich, Stephan
Amaro, Pedro
Andoche, Adrien
Baptista, Gonçalo
Bray, Connor
Cantor, Robin
Diercks, David
Fretwell, Spencer L.
Gillespie, Abigail
Hall, Ad
Harris, Cameron N.
Harris, Jackson T.
Hayen, Leendert M.
Hervieux, Paul Antoine
Indelicato, Paul
Kim, Geon Bo
Leach, Kyle G.
Lennarz, Annika
Lordi, Vincenzo
Machule, Peter
Marino, Andrew
McKeen, David
Mougeot, Xavier
Pinheiro, Daniel
Ponce, Francisco
Ruiz, Chris
Samanta, Amit
Santos, José Paulo
Smolsky, Joseph
Stone-Whitehead, Caitlyn
Templet, Joseph
Warburton, William K.
Waters, Benjamin
Machado, Jorge
Atomic Physics
The most stringent laboratory-based experimental limits on the existence of sub-MeV sterile neutrinos are currently set by decay spectroscopy of radioactive $^7$Be embedded into superconducting sensors. The systematic uncertainties are dominated by the modeling of the electron shake-up and shake-off spectra that are not based on state-of-the-art atomic theory and do not include electron correlations or relativistic effects. We have used the multiconfiguration Dirac-Fock formalism to obtain correlated wavefunctions ab initio and compute all single and double shake processes in the electron capture decay of atomic $^7$Be. The simulations can explain some but not all of the observed spectral features, likely because the wave functions are modified by the Ta sensor material that the $^7$Be is embedded into. The new models also show that the L/K electron capture ratio of $^7$Be in Ta has previously been slightly underestimated revising the previous value of 0.070(7) to a new value of 0.0756(20).
title Shake-up and shake-off spectra in the electron capture decay of atomic $^7$Be
topic Atomic Physics
url https://arxiv.org/abs/2601.16756