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Main Authors: Varshney, Harsh, Agarwal, Amit
Format: Preprint
Published: 2026
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Online Access:https://arxiv.org/abs/2601.17775
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author Varshney, Harsh
Agarwal, Amit
author_facet Varshney, Harsh
Agarwal, Amit
contents The nonlinear Nernst and Seebeck effects (NNE and NSE) offer promising routes for thermoelectric energy conversion in non-magnetic systems. While intrinsic mechanisms such as the nonlinear Drude and Berry-curvature-dipole terms are well established, extrinsic contributions to thermoelectric responses arising from disorder-induced asymmetric scattering remain comparatively less explored, despite growing experimental evidence of their dominance. Here, we develop a unified semiclassical theory of NNE and NSE that incorporates skew scattering and side-jump processes, identifying four distinct extrinsic contributions to NNE and two for NSE. A systematic symmetry analysis shows that these responses are allowed in time-reversal-symmetric non-magnets, PT-symmetric antiferromagnets, and non-centrosymmetric magnetic systems such as altermagnets. As a case study, we demonstrate that ABA-stacked trilayer graphene hosts large nonlinear Nernst and Seebeck responses dominated by extrinsic scattering, in excellent agreement with recent experiments. Our results establish the microscopic origin of these effects and provide guiding principles for designing high-efficiency nonlinear thermoelectric devices.
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publishDate 2026
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spellingShingle Asymmetric Scattering Drives Large Nonlinear Nernst and Seebeck Effects
Varshney, Harsh
Agarwal, Amit
Mesoscale and Nanoscale Physics
The nonlinear Nernst and Seebeck effects (NNE and NSE) offer promising routes for thermoelectric energy conversion in non-magnetic systems. While intrinsic mechanisms such as the nonlinear Drude and Berry-curvature-dipole terms are well established, extrinsic contributions to thermoelectric responses arising from disorder-induced asymmetric scattering remain comparatively less explored, despite growing experimental evidence of their dominance. Here, we develop a unified semiclassical theory of NNE and NSE that incorporates skew scattering and side-jump processes, identifying four distinct extrinsic contributions to NNE and two for NSE. A systematic symmetry analysis shows that these responses are allowed in time-reversal-symmetric non-magnets, PT-symmetric antiferromagnets, and non-centrosymmetric magnetic systems such as altermagnets. As a case study, we demonstrate that ABA-stacked trilayer graphene hosts large nonlinear Nernst and Seebeck responses dominated by extrinsic scattering, in excellent agreement with recent experiments. Our results establish the microscopic origin of these effects and provide guiding principles for designing high-efficiency nonlinear thermoelectric devices.
title Asymmetric Scattering Drives Large Nonlinear Nernst and Seebeck Effects
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2601.17775