Realization of a Wigner-Mott insulator in 6R-TaS$_2$ superconductor

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Hauptverfasser: Xiao, Hongqin, Li, Geng, He, Yuxuan, Zhu, Ke, Ye, Yuhan, Li, Yumeng, Huang, Lijing, Xiong, Pucen, Yang, Haitao, Wang, Ziqiang, Gao, Hong-Jun
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Veröffentlicht: 2026
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author Xiao, Hongqin
Li, Geng
He, Yuxuan
Zhu, Ke
Ye, Yuhan
Li, Yumeng
Huang, Lijing
Xiong, Pucen
Yang, Haitao
Wang, Ziqiang
Gao, Hong-Jun
author_facet Xiao, Hongqin
Li, Geng
He, Yuxuan
Zhu, Ke
Ye, Yuhan
Li, Yumeng
Huang, Lijing
Xiong, Pucen
Yang, Haitao
Wang, Ziqiang
Gao, Hong-Jun
contents Wigner-Mott insulating states represent a paradigmatic manifestation of strong electronic correlations, in which long-range Coulomb interactions drive spontaneous charge ordering and enable Mott localization at fractional electronic fillings. Such states have been theoretically proposed to arise from the cooperative interplay between onsite and inter-site Coulomb interactions. However, experimental realizations of the simultaneous microscopic observation of interaction-driven charge order and genuine Mott localization, which are the defining hallmarks of a Wigner-Mott insulator, have remained elusive. Here we report the observation of a Wigner-Mott insulating state in 6R-TaS$_2$ using scanning tunneling microscopy. By locally injecting electrons into the depleted 1T layer, we induce distinct Star-of-David charge-ordered superstructures and realize a cascade of insulating phases. In particular, a $\sqrt{3}\times \sqrt{3}$ charge-ordered superstructure at one-third filling hosts a robust Mott gap despite fractional filling. The spontaneous relaxation from excited states back to the ground state demonstrates that this Wigner-Mott phase is stabilized by the cooperative effects of onsite and inter-site Coulomb interactions. Our results provide direct microscopic evidence for a Wigner-Mott mechanism and establish 6R-TaS$_2$ as a platform for the controlled realization and investigation of Wigner-Mott insulating states.
format Preprint
id arxiv_https___arxiv_org_abs_2601_19482
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Realization of a Wigner-Mott insulator in 6R-TaS$_2$ superconductor
Xiao, Hongqin
Li, Geng
He, Yuxuan
Zhu, Ke
Ye, Yuhan
Li, Yumeng
Huang, Lijing
Xiong, Pucen
Yang, Haitao
Wang, Ziqiang
Gao, Hong-Jun
Strongly Correlated Electrons
Wigner-Mott insulating states represent a paradigmatic manifestation of strong electronic correlations, in which long-range Coulomb interactions drive spontaneous charge ordering and enable Mott localization at fractional electronic fillings. Such states have been theoretically proposed to arise from the cooperative interplay between onsite and inter-site Coulomb interactions. However, experimental realizations of the simultaneous microscopic observation of interaction-driven charge order and genuine Mott localization, which are the defining hallmarks of a Wigner-Mott insulator, have remained elusive. Here we report the observation of a Wigner-Mott insulating state in 6R-TaS$_2$ using scanning tunneling microscopy. By locally injecting electrons into the depleted 1T layer, we induce distinct Star-of-David charge-ordered superstructures and realize a cascade of insulating phases. In particular, a $\sqrt{3}\times \sqrt{3}$ charge-ordered superstructure at one-third filling hosts a robust Mott gap despite fractional filling. The spontaneous relaxation from excited states back to the ground state demonstrates that this Wigner-Mott phase is stabilized by the cooperative effects of onsite and inter-site Coulomb interactions. Our results provide direct microscopic evidence for a Wigner-Mott mechanism and establish 6R-TaS$_2$ as a platform for the controlled realization and investigation of Wigner-Mott insulating states.
title Realization of a Wigner-Mott insulator in 6R-TaS$_2$ superconductor
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2601.19482