All-electrical switching of spin texture in a strain-tunable 2D Janus ferroelectric altermagnet

Fuente: arXiv
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Auteurs principaux: Yao, Tao, Shen, Quan, Liao, Wenhu, Tan, Jianing, Dong, Jiansheng
Format: Preprint
Publié: 2026
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author Yao, Tao
Shen, Quan
Liao, Wenhu
Tan, Jianing
Dong, Jiansheng
author_facet Yao, Tao
Shen, Quan
Liao, Wenhu
Tan, Jianing
Dong, Jiansheng
contents Altermagnetism (AM), a collinear magnetic phase with momentum-dependent spin splitting, is a promising candidate for strong magnetoelectric coupling. However, realizing direct and tunable coupling between ferroelectricity (FE) and AM within a single two-dimensional (2D) material remains an outstanding challenge. Here, based on first-principles calculations, we identify the distorted phase of monolayer Janus VOClBr as an intrinsic 2D FE-AM. This phase demonstrates robust magnetoelectric coupling, as evidenced by a complete reversal of momentum-space spin polarization upon FE switching, and further supported by spin texture analysis and the magneto-optical Kerr effect. Notably, the FE properties are highly strain-tunable: biaxial compression strain of -4% reduces the FE polarization switching barrier by approximately 87%, whereas a tensile strain of +3% induces a phase transition to an antiferromagnet. Leveraging the lock-in between the electrically controlled spin texture and the magneto-optical Kerr effect signal, we propose a non-volatile, polymorphic spintronic memory device featuring all-electrical writing and optical readout. This work establishes 2D FE-AMs as a versatile platform for coupled ferroic orders and paves the way for voltage-controlled, multifunctional spin-logic devices.
format Preprint
id arxiv_https___arxiv_org_abs_2601_19560
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle All-electrical switching of spin texture in a strain-tunable 2D Janus ferroelectric altermagnet
Yao, Tao
Shen, Quan
Liao, Wenhu
Tan, Jianing
Dong, Jiansheng
Materials Science
Mesoscale and Nanoscale Physics
Altermagnetism (AM), a collinear magnetic phase with momentum-dependent spin splitting, is a promising candidate for strong magnetoelectric coupling. However, realizing direct and tunable coupling between ferroelectricity (FE) and AM within a single two-dimensional (2D) material remains an outstanding challenge. Here, based on first-principles calculations, we identify the distorted phase of monolayer Janus VOClBr as an intrinsic 2D FE-AM. This phase demonstrates robust magnetoelectric coupling, as evidenced by a complete reversal of momentum-space spin polarization upon FE switching, and further supported by spin texture analysis and the magneto-optical Kerr effect. Notably, the FE properties are highly strain-tunable: biaxial compression strain of -4% reduces the FE polarization switching barrier by approximately 87%, whereas a tensile strain of +3% induces a phase transition to an antiferromagnet. Leveraging the lock-in between the electrically controlled spin texture and the magneto-optical Kerr effect signal, we propose a non-volatile, polymorphic spintronic memory device featuring all-electrical writing and optical readout. This work establishes 2D FE-AMs as a versatile platform for coupled ferroic orders and paves the way for voltage-controlled, multifunctional spin-logic devices.
title All-electrical switching of spin texture in a strain-tunable 2D Janus ferroelectric altermagnet
topic Materials Science
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2601.19560