Fundamental Relations as the Leading Order in Nonlinear Thermoelectric Responses with Time-Reversal Symmetry

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Hauptverfasser: Zhang, Ying-Fei, Zhang, Zhi-Fan, Jiang, Hua, Zhu, Zhen-Gang, Su, Gang
Format: Preprint
Veröffentlicht: 2026
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author Zhang, Ying-Fei
Zhang, Zhi-Fan
Jiang, Hua
Zhu, Zhen-Gang
Su, Gang
author_facet Zhang, Ying-Fei
Zhang, Zhi-Fan
Jiang, Hua
Zhu, Zhen-Gang
Su, Gang
contents In recent years, nonlinear transport phenomena have garnered significant interest in both theoretical explorations and experiments. In this work, we utilize the semi-classical wave packet theory to calculate disorder-induced second-order transport coefficients: second-order electrical ($σ$), thermoelectric ($α$), and thermal ($κ$) coefficients, capturing the interplay between side-jump and skew-scattering contributions in systems with time-reversal symmetry. Using a topological insulator model, we quantitatively characterize the Fermi-level dependence of these second-order transport coefficients by explicitly including Coulomb impurity potentials. Furthermore, we elucidate the relationships between these coefficients, establishing the second-order Mott relation and the Wiedemann-Franz law induced by disorder. This study develops a comprehensive theoretical framework elucidating the nonlinear thermoelectric transport mechanisms in quantum material systems.
format Preprint
id arxiv_https___arxiv_org_abs_2601_19625
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Fundamental Relations as the Leading Order in Nonlinear Thermoelectric Responses with Time-Reversal Symmetry
Zhang, Ying-Fei
Zhang, Zhi-Fan
Jiang, Hua
Zhu, Zhen-Gang
Su, Gang
Mesoscale and Nanoscale Physics
In recent years, nonlinear transport phenomena have garnered significant interest in both theoretical explorations and experiments. In this work, we utilize the semi-classical wave packet theory to calculate disorder-induced second-order transport coefficients: second-order electrical ($σ$), thermoelectric ($α$), and thermal ($κ$) coefficients, capturing the interplay between side-jump and skew-scattering contributions in systems with time-reversal symmetry. Using a topological insulator model, we quantitatively characterize the Fermi-level dependence of these second-order transport coefficients by explicitly including Coulomb impurity potentials. Furthermore, we elucidate the relationships between these coefficients, establishing the second-order Mott relation and the Wiedemann-Franz law induced by disorder. This study develops a comprehensive theoretical framework elucidating the nonlinear thermoelectric transport mechanisms in quantum material systems.
title Fundamental Relations as the Leading Order in Nonlinear Thermoelectric Responses with Time-Reversal Symmetry
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2601.19625