Tunable Nanoparticle Stripe Patterns at Inclined Surfaces

Fuente: arXiv
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Autori principali: Bhattacharjee, Suman, Khawas, Sanjoy, Srivastava, Sunita
Natura: Preprint
Pubblicazione: 2026
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author Bhattacharjee, Suman
Khawas, Sanjoy
Srivastava, Sunita
author_facet Bhattacharjee, Suman
Khawas, Sanjoy
Srivastava, Sunita
contents Periodic assemblies of nanoparticles are central to surface patterning, with applications in biosensing, energy conversion, and nanofabrication. Evaporation of colloidal droplets on substrates provides a simple yet effective route to achieve such assemblies. This work reports the first experimental demonstration of patterns formed through stick-slip dynamics of the three-phase contact line during evaporation of gold nanoparticle suspensions on inclined substrates. Variation in nanoparticle concentration and substrate inclination alter the balance of interfacial and gravitational forces, producing multiple stick-slip events that generate periodic stripes. Stripe density exhibits a sinusoidal dependence on inclination angle, while inter-stripe spacing remains nearly invariant. Independent control over inter-stripe spacing is achieved through adjustment of nanoparticle or surfactant concentration. These results highlight the complex interplay of gravitational and interfacial forces in directing periodic nanoparticle assembly and establish a versatile, programmable framework for surface patterning with tunable nano/microscale dimensions.
format Preprint
id arxiv_https___arxiv_org_abs_2601_20165
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Tunable Nanoparticle Stripe Patterns at Inclined Surfaces
Bhattacharjee, Suman
Khawas, Sanjoy
Srivastava, Sunita
Soft Condensed Matter
Mesoscale and Nanoscale Physics
Materials Science
Periodic assemblies of nanoparticles are central to surface patterning, with applications in biosensing, energy conversion, and nanofabrication. Evaporation of colloidal droplets on substrates provides a simple yet effective route to achieve such assemblies. This work reports the first experimental demonstration of patterns formed through stick-slip dynamics of the three-phase contact line during evaporation of gold nanoparticle suspensions on inclined substrates. Variation in nanoparticle concentration and substrate inclination alter the balance of interfacial and gravitational forces, producing multiple stick-slip events that generate periodic stripes. Stripe density exhibits a sinusoidal dependence on inclination angle, while inter-stripe spacing remains nearly invariant. Independent control over inter-stripe spacing is achieved through adjustment of nanoparticle or surfactant concentration. These results highlight the complex interplay of gravitational and interfacial forces in directing periodic nanoparticle assembly and establish a versatile, programmable framework for surface patterning with tunable nano/microscale dimensions.
title Tunable Nanoparticle Stripe Patterns at Inclined Surfaces
topic Soft Condensed Matter
Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2601.20165