Magnetic states of the Kondo lattice Ce$_2$PdSi$_3$ and their pressure evolution

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Hauptverfasser: Zhang, Yanan, Shan, Zhaoyang, Zhang, Jiawen, Ye, Kaixin, Li, Yongjian, Su, Dajun, Manuel, Pascal, Khalyavin, Dmitry, Adroja, Devashibhai, Mayoh, Daniel, Balakrishnan, Geetha, Liu, Yu, Smidman, Michael, Yuan, Huiqiu
Format: Preprint
Veröffentlicht: 2026
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author Zhang, Yanan
Shan, Zhaoyang
Zhang, Jiawen
Ye, Kaixin
Li, Yongjian
Su, Dajun
Manuel, Pascal
Khalyavin, Dmitry
Adroja, Devashibhai
Mayoh, Daniel
Balakrishnan, Geetha
Liu, Yu
Smidman, Michael
Yuan, Huiqiu
author_facet Zhang, Yanan
Shan, Zhaoyang
Zhang, Jiawen
Ye, Kaixin
Li, Yongjian
Su, Dajun
Manuel, Pascal
Khalyavin, Dmitry
Adroja, Devashibhai
Mayoh, Daniel
Balakrishnan, Geetha
Liu, Yu
Smidman, Michael
Yuan, Huiqiu
contents Frustrated Kondo lattices are ideal platforms for exploring unconventional forms of quantum criticality, as well as magnetism and other emergent phases. Here we report the magnetic properties of the candidate frustrated heavy fermion compound Ce$_2$PdSi$_3$, and map their evolution upon applying magnetic fields and hydrostatic pressure. We find that at ambient pressure Ce$_2$PdSi$_3$ exhibits two distinct magnetic phase transitions, a ferromagnetic-like transition at $T_{\mathrm{M1}}=3.8$ K and an incommensurate antiferromagnetic transition at $T_{\mathrm{M2}}=2.9$ K. Upon applying pressure, $T_{\mathrm{M1}}$ is continuously suppressed and becomes undetectable above 4.2 GPa, whereas $T_{\mathrm{M2}}$ increases and remains robust up to at least 7.5 GPa. The observed pressure evolution of magnetic order in Ce$_2$PdSi$_3$ suggests the presence of competing magnetic orders, and cannot be simply encapsulated by the Doniach phase diagram, motivating further investigations for its origin, including discerning the role of geometric frustration.
format Preprint
id arxiv_https___arxiv_org_abs_2601_20517
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Magnetic states of the Kondo lattice Ce$_2$PdSi$_3$ and their pressure evolution
Zhang, Yanan
Shan, Zhaoyang
Zhang, Jiawen
Ye, Kaixin
Li, Yongjian
Su, Dajun
Manuel, Pascal
Khalyavin, Dmitry
Adroja, Devashibhai
Mayoh, Daniel
Balakrishnan, Geetha
Liu, Yu
Smidman, Michael
Yuan, Huiqiu
Strongly Correlated Electrons
Frustrated Kondo lattices are ideal platforms for exploring unconventional forms of quantum criticality, as well as magnetism and other emergent phases. Here we report the magnetic properties of the candidate frustrated heavy fermion compound Ce$_2$PdSi$_3$, and map their evolution upon applying magnetic fields and hydrostatic pressure. We find that at ambient pressure Ce$_2$PdSi$_3$ exhibits two distinct magnetic phase transitions, a ferromagnetic-like transition at $T_{\mathrm{M1}}=3.8$ K and an incommensurate antiferromagnetic transition at $T_{\mathrm{M2}}=2.9$ K. Upon applying pressure, $T_{\mathrm{M1}}$ is continuously suppressed and becomes undetectable above 4.2 GPa, whereas $T_{\mathrm{M2}}$ increases and remains robust up to at least 7.5 GPa. The observed pressure evolution of magnetic order in Ce$_2$PdSi$_3$ suggests the presence of competing magnetic orders, and cannot be simply encapsulated by the Doniach phase diagram, motivating further investigations for its origin, including discerning the role of geometric frustration.
title Magnetic states of the Kondo lattice Ce$_2$PdSi$_3$ and their pressure evolution
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2601.20517