Intersubband electric dipole spin resonance in transition metal dichalcogenide heterobilayers

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Hauptverfasser: Grigoryan, K. K., Glazov, M. M.
Format: Preprint
Veröffentlicht: 2026
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author Grigoryan, K. K.
Glazov, M. M.
author_facet Grigoryan, K. K.
Glazov, M. M.
contents The theory of inter-spin-subband electric dipole spin resonance in transition metal dichalcogenide heterobilayers is proposed. Our symmetry analysis demonstrates that, in contrast to monolayers, the reduced symmetry of heterobilayers enables coupling between conduction band spin subbands by an electric field. We establish the optical selection rules for all six high-symmetry stacking configurations. The microscopic mechanism of the effect is identified as the spin-orbit coupling induced mixing of Bloch states from different conduction bands, which generates a non-zero momentum matrix element between the spin-split states. It also leads to the linear-in-wavevector spin-dependent terms in the effective Hamiltonian, i.e., the Rashba effect. Our estimates show that the rate of electric-dipole spin-flip transitions exceeds by far that of the magnetic-dipole transitions in transition metal dichalcogenide heterobilayers.
format Preprint
id arxiv_https___arxiv_org_abs_2602_02111
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Intersubband electric dipole spin resonance in transition metal dichalcogenide heterobilayers
Grigoryan, K. K.
Glazov, M. M.
Mesoscale and Nanoscale Physics
Materials Science
Other Condensed Matter
The theory of inter-spin-subband electric dipole spin resonance in transition metal dichalcogenide heterobilayers is proposed. Our symmetry analysis demonstrates that, in contrast to monolayers, the reduced symmetry of heterobilayers enables coupling between conduction band spin subbands by an electric field. We establish the optical selection rules for all six high-symmetry stacking configurations. The microscopic mechanism of the effect is identified as the spin-orbit coupling induced mixing of Bloch states from different conduction bands, which generates a non-zero momentum matrix element between the spin-split states. It also leads to the linear-in-wavevector spin-dependent terms in the effective Hamiltonian, i.e., the Rashba effect. Our estimates show that the rate of electric-dipole spin-flip transitions exceeds by far that of the magnetic-dipole transitions in transition metal dichalcogenide heterobilayers.
title Intersubband electric dipole spin resonance in transition metal dichalcogenide heterobilayers
topic Mesoscale and Nanoscale Physics
Materials Science
Other Condensed Matter
url https://arxiv.org/abs/2602.02111