Quasi-one-dimensional spin excitations in the iron pnictide NaFe$_{0.53}$Cu$_{0.47}$As

Fuente: arXiv
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Autori principali: Wang, Yifan, Tam, David W., Wang, Weiyi, Ewings, R. A., Stewart, J. Ross, Matsuda, Masaaki, Cao, Chongde, Liu, Changle, Yu, Rong, Dai, Pengcheng, Song, Yu
Natura: Preprint
Pubblicazione: 2026
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author Wang, Yifan
Tam, David W.
Wang, Weiyi
Ewings, R. A.
Stewart, J. Ross
Matsuda, Masaaki
Cao, Chongde
Liu, Changle
Yu, Rong
Dai, Pengcheng
Song, Yu
author_facet Wang, Yifan
Tam, David W.
Wang, Weiyi
Ewings, R. A.
Stewart, J. Ross
Matsuda, Masaaki
Cao, Chongde
Liu, Changle
Yu, Rong
Dai, Pengcheng
Song, Yu
contents Spectroscopic measurements in model one-dimensional (1D) correlated systems offer insights for understanding their two-dimensional counterparts, which include the cuprate and iron pnictide/chalcogenide superconductors. A major challenge is the identification of such correlated systems with dominantly 1D physics. In this work, inelastic neutron scattering measurements on NaFe$_{0.53}$Cu$_{0.47}$As single crystal directly reveal quasi-1D spin excitations, resulting from atomic order that lead to magnetic Fe and nonmagnetic Cu chains. The dominant exchange interaction is antiferromagnetic along the chain ($SJ_{\rm \parallel}\approx90.1(3)$~meV), whereas the inter-chain couplings are much weaker ($SJ_{\rm \perp}\approx-2.4(1)$~meV and $SJ_{\rm c}\approx0.15(5)$~meV). The quasi-1D spin excitations in NaFe$_{0.53}$Cu$_{0.47}$As stem from both the Néel and stripe vectors, with Néel excitations sensitive to Fe impurities on the Cu site. The spin excitations in quasi-1D NaFe$_{0.53}$Cu$_{0.47}$As and quasi-2D FeSe exhibit a striking resemblance, suggesting a common origin for their coexistent stripe and Néel excitations. Our findings demonstrate magnetic dilution in NaFeAs leads to dimension reduction of its magnetic degree of freedom, presenting a strategy for discovering low-dimensional quantum materials.
format Preprint
id arxiv_https___arxiv_org_abs_2602_06705
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Quasi-one-dimensional spin excitations in the iron pnictide NaFe$_{0.53}$Cu$_{0.47}$As
Wang, Yifan
Tam, David W.
Wang, Weiyi
Ewings, R. A.
Stewart, J. Ross
Matsuda, Masaaki
Cao, Chongde
Liu, Changle
Yu, Rong
Dai, Pengcheng
Song, Yu
Strongly Correlated Electrons
Spectroscopic measurements in model one-dimensional (1D) correlated systems offer insights for understanding their two-dimensional counterparts, which include the cuprate and iron pnictide/chalcogenide superconductors. A major challenge is the identification of such correlated systems with dominantly 1D physics. In this work, inelastic neutron scattering measurements on NaFe$_{0.53}$Cu$_{0.47}$As single crystal directly reveal quasi-1D spin excitations, resulting from atomic order that lead to magnetic Fe and nonmagnetic Cu chains. The dominant exchange interaction is antiferromagnetic along the chain ($SJ_{\rm \parallel}\approx90.1(3)$~meV), whereas the inter-chain couplings are much weaker ($SJ_{\rm \perp}\approx-2.4(1)$~meV and $SJ_{\rm c}\approx0.15(5)$~meV). The quasi-1D spin excitations in NaFe$_{0.53}$Cu$_{0.47}$As stem from both the Néel and stripe vectors, with Néel excitations sensitive to Fe impurities on the Cu site. The spin excitations in quasi-1D NaFe$_{0.53}$Cu$_{0.47}$As and quasi-2D FeSe exhibit a striking resemblance, suggesting a common origin for their coexistent stripe and Néel excitations. Our findings demonstrate magnetic dilution in NaFeAs leads to dimension reduction of its magnetic degree of freedom, presenting a strategy for discovering low-dimensional quantum materials.
title Quasi-one-dimensional spin excitations in the iron pnictide NaFe$_{0.53}$Cu$_{0.47}$As
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2602.06705