Hyperfine interaction of electrons and holes with nuclei probed by optical orientation in MAPbI$_3$ perovskite crystals

Fuente: arXiv
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Autores principales: Kotur, Mladen, Kopteva, Nataliia E., Yakovlev, Dmitri R., Turedi, Bekir, Kovalenko, Maksym V., Bayer, Manfred
Formato: Preprint
Publicado: 2026
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author Kotur, Mladen
Kopteva, Nataliia E.
Yakovlev, Dmitri R.
Turedi, Bekir
Kovalenko, Maksym V.
Bayer, Manfred
author_facet Kotur, Mladen
Kopteva, Nataliia E.
Yakovlev, Dmitri R.
Turedi, Bekir
Kovalenko, Maksym V.
Bayer, Manfred
contents Optical orientation of electron and hole spins by circularly polarized light is investigated for MAPbI$_3$ single crystals. The Hanle and polarization recovery effects measured in transverse and longitudinal magnetic fields, respectively, evidence the hyperfine interaction with nuclear spins as the main factor determining the spin dynamics of charge carriers at cryogenic temperatures. The parameters of the nuclear spin fluctuations within the carrier localization volume are evaluated. Dynamic polarization of the nuclear spins is demonstrated by the Overhauser field reaching 5 mT for acting on the electrons and -30 mT for acting on the holes.
format Preprint
id arxiv_https___arxiv_org_abs_2602_07691
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Hyperfine interaction of electrons and holes with nuclei probed by optical orientation in MAPbI$_3$ perovskite crystals
Kotur, Mladen
Kopteva, Nataliia E.
Yakovlev, Dmitri R.
Turedi, Bekir
Kovalenko, Maksym V.
Bayer, Manfred
Mesoscale and Nanoscale Physics
Optical orientation of electron and hole spins by circularly polarized light is investigated for MAPbI$_3$ single crystals. The Hanle and polarization recovery effects measured in transverse and longitudinal magnetic fields, respectively, evidence the hyperfine interaction with nuclear spins as the main factor determining the spin dynamics of charge carriers at cryogenic temperatures. The parameters of the nuclear spin fluctuations within the carrier localization volume are evaluated. Dynamic polarization of the nuclear spins is demonstrated by the Overhauser field reaching 5 mT for acting on the electrons and -30 mT for acting on the holes.
title Hyperfine interaction of electrons and holes with nuclei probed by optical orientation in MAPbI$_3$ perovskite crystals
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2602.07691