Terahertz Synthetic FM Triplet for Distortion-Free Stabilization and Lamb-Dip Spectroscopy

Fuente: arXiv
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Autores principales: Eguchi, Kohei, Tanaka, Toki, Ito, Hiroshi, Tanaka, Koichiro
Formato: Preprint
Publicado: 2026
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author Eguchi, Kohei
Tanaka, Toki
Ito, Hiroshi
Tanaka, Koichiro
author_facet Eguchi, Kohei
Tanaka, Toki
Ito, Hiroshi
Tanaka, Koichiro
contents We demonstrate a distortion-free terahertz frequency stabilization technique using a "synthetic FM triplet" to overcome modulation sideband interference associated with high-density spectral lines in molecular clocks. By applying this method to the rotational transitions of acetonitrile (CH$_3$CN), we successfully generated clean derivative waveforms free from inter-line interference, achieving a fractional frequency instability of $1 \times 10^{-9}$ at an averaging time of $1~\mathrm{s}$. Furthermore, we report the observation of Lamb-dips using this high-fidelity approach. Our results establish acetonitrile as a promising candidate for high-agility molecular clocks and provide a robust solution for precision spectroscopy of molecules with complex hyperfine structures.
format Preprint
id arxiv_https___arxiv_org_abs_2602_07737
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Terahertz Synthetic FM Triplet for Distortion-Free Stabilization and Lamb-Dip Spectroscopy
Eguchi, Kohei
Tanaka, Toki
Ito, Hiroshi
Tanaka, Koichiro
Optics
We demonstrate a distortion-free terahertz frequency stabilization technique using a "synthetic FM triplet" to overcome modulation sideband interference associated with high-density spectral lines in molecular clocks. By applying this method to the rotational transitions of acetonitrile (CH$_3$CN), we successfully generated clean derivative waveforms free from inter-line interference, achieving a fractional frequency instability of $1 \times 10^{-9}$ at an averaging time of $1~\mathrm{s}$. Furthermore, we report the observation of Lamb-dips using this high-fidelity approach. Our results establish acetonitrile as a promising candidate for high-agility molecular clocks and provide a robust solution for precision spectroscopy of molecules with complex hyperfine structures.
title Terahertz Synthetic FM Triplet for Distortion-Free Stabilization and Lamb-Dip Spectroscopy
topic Optics
url https://arxiv.org/abs/2602.07737