Frustrated spin models on two- and three-dimensional decorated lattices with high residual entropy

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Main Authors: Dmitriev, D. V., Krivnov, V. Ya., Vasilyev, O. A.
Format: Preprint
Published: 2026
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author Dmitriev, D. V.
Krivnov, V. Ya.
Vasilyev, O. A.
author_facet Dmitriev, D. V.
Krivnov, V. Ya.
Vasilyev, O. A.
contents We study the ground-state properties of a family of frustrated spin-1/2 Heisenberg models on two- and three-dimensional decorated lattices composed of connected star-shaped units. Each star is built from edge-sharing triangles with an antiferromagnetic interaction on the shared side and ferromagnetic interactions on the others. At a critical coupling ratio, the ideal star model - defined by equal ferromagnetic interactions - exhibits a macroscopically degenerate ground state, which we map onto a site percolation problem on the Lieb lattice. This mapping enables the calculation of exponential ground-state degeneracy and the corresponding residual entropy for square, triangular, honeycomb, and cubic lattices. Remarkably, the residual entropy remains high for all studied lattices, exceeding 60\% of the maximal value ln(2). Despite a gapless quadratic one-magnon spectrum, the low-temperature thermodynamics is governed by exponentially numerous gapped excitations. For a distorted-star variant of the model, the ground-state manifold is equivalent to that of decoupled ferromagnetic clusters, leading to exponential degeneracy with a lower, yet still substantial, residual entropy. At low temperature the system mimics a paramagnetic crystal of non-interacting spins with high spin value ($s=4$ for a square lattice). The obtained results establish a structural design principle for engineering quantum magnets with a high ground-state degeneracy, suggesting promising candidates for enhanced magnetocaloric cooling and quantum thermal machines.
format Preprint
id arxiv_https___arxiv_org_abs_2602_08674
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Frustrated spin models on two- and three-dimensional decorated lattices with high residual entropy
Dmitriev, D. V.
Krivnov, V. Ya.
Vasilyev, O. A.
Strongly Correlated Electrons
Statistical Mechanics
We study the ground-state properties of a family of frustrated spin-1/2 Heisenberg models on two- and three-dimensional decorated lattices composed of connected star-shaped units. Each star is built from edge-sharing triangles with an antiferromagnetic interaction on the shared side and ferromagnetic interactions on the others. At a critical coupling ratio, the ideal star model - defined by equal ferromagnetic interactions - exhibits a macroscopically degenerate ground state, which we map onto a site percolation problem on the Lieb lattice. This mapping enables the calculation of exponential ground-state degeneracy and the corresponding residual entropy for square, triangular, honeycomb, and cubic lattices. Remarkably, the residual entropy remains high for all studied lattices, exceeding 60\% of the maximal value ln(2). Despite a gapless quadratic one-magnon spectrum, the low-temperature thermodynamics is governed by exponentially numerous gapped excitations. For a distorted-star variant of the model, the ground-state manifold is equivalent to that of decoupled ferromagnetic clusters, leading to exponential degeneracy with a lower, yet still substantial, residual entropy. At low temperature the system mimics a paramagnetic crystal of non-interacting spins with high spin value ($s=4$ for a square lattice). The obtained results establish a structural design principle for engineering quantum magnets with a high ground-state degeneracy, suggesting promising candidates for enhanced magnetocaloric cooling and quantum thermal machines.
title Frustrated spin models on two- and three-dimensional decorated lattices with high residual entropy
topic Strongly Correlated Electrons
Statistical Mechanics
url https://arxiv.org/abs/2602.08674