Three-dimensional real-space electron dynamics in graphene driven by strong laser fields

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Bibliographic Details
Main Authors:	Li, S., Tani, M., Hashmi, A., Ishikawa, K. L.
Format:	Preprint
Published:	2026
Subjects:	Mesoscale and Nanoscale Physics
Online Access:	Acceder al recurso
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author	Li, S. Tani, M. Hashmi, A. Ishikawa, K. L.
author_facet	Li, S. Tani, M. Hashmi, A. Ishikawa, K. L.
contents	We theoretically investigate the three-dimensional (3D) electron dynamics of graphene in real space under strong laser fields using time-dependent density functional theory (TDDFT). We successfully reproduce the reversal of current direction originating from the cancellation of two oppositely directed residual currents, as previously predicted by Morimoto et al. [Y. Morimoto et al., New J. Phys. 24, 033051 (2022)]. By distinguishing contributions from individual orbitals, our results validate the two-level system approximation and also emphasize that the first-principles approach agrees better with experimental results for light-driven residual current, especially in extremely strong fields. Furthermore, our 3D model reveals that the real-space atomic-scale current induced by strong laser fields is concentrated slightly above and below the graphene basal plane, rather than strictly within it. The two oppositely directed currents exhibit a pronounced height separation in the out-of-plane direction, indicating that the ring current is not confined to the graphene plane but forms a rotating 3D circulation loop which is absent in the reduced-dimensional model.
format	Preprint
id	arxiv_https___arxiv_org_abs_2602_09440
institution	arXiv
publishDate	2026
record_format	arxiv
spellingShingle	Three-dimensional real-space electron dynamics in graphene driven by strong laser fields Li, S. Tani, M. Hashmi, A. Ishikawa, K. L. Mesoscale and Nanoscale Physics We theoretically investigate the three-dimensional (3D) electron dynamics of graphene in real space under strong laser fields using time-dependent density functional theory (TDDFT). We successfully reproduce the reversal of current direction originating from the cancellation of two oppositely directed residual currents, as previously predicted by Morimoto et al. [Y. Morimoto et al., New J. Phys. 24, 033051 (2022)]. By distinguishing contributions from individual orbitals, our results validate the two-level system approximation and also emphasize that the first-principles approach agrees better with experimental results for light-driven residual current, especially in extremely strong fields. Furthermore, our 3D model reveals that the real-space atomic-scale current induced by strong laser fields is concentrated slightly above and below the graphene basal plane, rather than strictly within it. The two oppositely directed currents exhibit a pronounced height separation in the out-of-plane direction, indicating that the ring current is not confined to the graphene plane but forms a rotating 3D circulation loop which is absent in the reduced-dimensional model.
title	Three-dimensional real-space electron dynamics in graphene driven by strong laser fields
topic	Mesoscale and Nanoscale Physics
url	https://arxiv.org/abs/2602.09440

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