Extending numerical simulations in SIMPSON: Electron paramagnetic resonance, dynamic nuclear polarisation, propagator splitting, pulse transients, and quadrupolar cross terms

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Auteurs principaux: Goodwin, David L., Carvalho, Jose P., Nielsen, Anders B., Wili, Nino, Vosegaard, Thomas, Tosner, Zdenek, Nielsen, Niels Chr.
Format: Preprint
Publié: 2026
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author Goodwin, David L.
Carvalho, Jose P.
Nielsen, Anders B.
Wili, Nino
Vosegaard, Thomas
Tosner, Zdenek
Nielsen, Niels Chr.
author_facet Goodwin, David L.
Carvalho, Jose P.
Nielsen, Anders B.
Wili, Nino
Vosegaard, Thomas
Tosner, Zdenek
Nielsen, Niels Chr.
contents Aimed at the simulation, design, and interpretation of advanced pulse experiments crossing the boundaries between nuclear magnetic resonance (NMR) and electron paramagnetic resonance (EPR), including the rapidly emerging, hybrid discipline of pulsed dynamic nuclear polarisation (DNP), we present a host of novel features in the widely used SIMPSON software package addressing these aspects. Along with this come new features for advanced pulse sequence evaluation in terms of propagator splitting, high-order spin operator cross terms, and pulse phase transients. These fundamental new tools are introduced in a C++-based next generation of the SIMPSON software, which improves calculations speed in some aspects, is better prepared for further developments, and facilitates easier community contributions to the open-source software package.
format Preprint
id arxiv_https___arxiv_org_abs_2602_15793
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Extending numerical simulations in SIMPSON: Electron paramagnetic resonance, dynamic nuclear polarisation, propagator splitting, pulse transients, and quadrupolar cross terms
Goodwin, David L.
Carvalho, Jose P.
Nielsen, Anders B.
Wili, Nino
Vosegaard, Thomas
Tosner, Zdenek
Nielsen, Niels Chr.
Chemical Physics
Aimed at the simulation, design, and interpretation of advanced pulse experiments crossing the boundaries between nuclear magnetic resonance (NMR) and electron paramagnetic resonance (EPR), including the rapidly emerging, hybrid discipline of pulsed dynamic nuclear polarisation (DNP), we present a host of novel features in the widely used SIMPSON software package addressing these aspects. Along with this come new features for advanced pulse sequence evaluation in terms of propagator splitting, high-order spin operator cross terms, and pulse phase transients. These fundamental new tools are introduced in a C++-based next generation of the SIMPSON software, which improves calculations speed in some aspects, is better prepared for further developments, and facilitates easier community contributions to the open-source software package.
title Extending numerical simulations in SIMPSON: Electron paramagnetic resonance, dynamic nuclear polarisation, propagator splitting, pulse transients, and quadrupolar cross terms
topic Chemical Physics
url https://arxiv.org/abs/2602.15793