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Bibliographic Details
Main Authors: Laskaris, G., Morozov, D., Tarpanov, D., Seth, A., Procelewska, J., Gautam, G. Sai, Sagingalieva, A., Brasher, R., Melnikov, A.
Format: Preprint
Published: 2026
Subjects:
Online Access:https://arxiv.org/abs/2602.16908
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Table of Contents:
  • Allegro is a machine learning interatomic potential (MLIP) model designed to predict atomic properties in molecules using E(3) equivariant neural networks. When training this model, there tends to be a trade-off between accuracy and inference time. For this reason we apply multi-objective hyperparameter optimization to the two objectives. Additionally, we experiment with modified architectures by making variants of Allegro some by adding strictly classical multi-layer perceptron (MLP) layers and some by adding quantum-classical hybrid layers. We compare the results from QM9, rMD17-aspirin, rMD17-benzene and our own proprietary dataset consisting of copper and lithium atoms. As results, we have a list of variants that surpass the Allegro in accuracy and also results which demonstrate the trade-off with inference times.