Reconfigurable Geometric Phase Matching by Multilayered Nonlinear Thin-Film Crystals

Fuente: arXiv
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Autori principali: Ben-Haim, Danielle, Tal, Mai, Xu, Xiaoxi, Ellenbogen, Tal
Natura: Preprint
Pubblicazione: 2026
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author Ben-Haim, Danielle
Tal, Mai
Xu, Xiaoxi
Ellenbogen, Tal
author_facet Ben-Haim, Danielle
Tal, Mai
Xu, Xiaoxi
Ellenbogen, Tal
contents Phase matching is essential for efficient energy transfer in nonlinear wave-mixing processes. Traditional methods, such as birefringent and quasi-phase matching, have remained conceptually unchanged since their discovery over 60 years ago, each posing inherent constraints and limitations. Here, we demonstrate the concept of geometric phase matching as a new paradigm for tunable nonlinear wave mixing, based on a multilayered platform of nonlinear thin-film crystals. We leverage this concept to experimentally show reconfigurable and spin-controlled phase matching for second-harmonic generation (SHG), opening new avenues for real-time manipulation of nonlinear interactions in photonic devices. We specifically demonstrate full modulation of SHG from a bilayer structure, nearly perfect and tunable geometric phase matching from an eight-layer structure, and polarization tomography that reveals the evolution of the spin dependent interaction. This approach not only expands the design space for nonlinear optical processes but also paves the way for highly robust, tunable and efficient frequency conversion, for next-generation adaptive nonlinear photonic, quantum photonic and nonlinear optical metamaterial technologies based on thin-film crystals.
format Preprint
id arxiv_https___arxiv_org_abs_2602_18418
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Reconfigurable Geometric Phase Matching by Multilayered Nonlinear Thin-Film Crystals
Ben-Haim, Danielle
Tal, Mai
Xu, Xiaoxi
Ellenbogen, Tal
Optics
Phase matching is essential for efficient energy transfer in nonlinear wave-mixing processes. Traditional methods, such as birefringent and quasi-phase matching, have remained conceptually unchanged since their discovery over 60 years ago, each posing inherent constraints and limitations. Here, we demonstrate the concept of geometric phase matching as a new paradigm for tunable nonlinear wave mixing, based on a multilayered platform of nonlinear thin-film crystals. We leverage this concept to experimentally show reconfigurable and spin-controlled phase matching for second-harmonic generation (SHG), opening new avenues for real-time manipulation of nonlinear interactions in photonic devices. We specifically demonstrate full modulation of SHG from a bilayer structure, nearly perfect and tunable geometric phase matching from an eight-layer structure, and polarization tomography that reveals the evolution of the spin dependent interaction. This approach not only expands the design space for nonlinear optical processes but also paves the way for highly robust, tunable and efficient frequency conversion, for next-generation adaptive nonlinear photonic, quantum photonic and nonlinear optical metamaterial technologies based on thin-film crystals.
title Reconfigurable Geometric Phase Matching by Multilayered Nonlinear Thin-Film Crystals
topic Optics
url https://arxiv.org/abs/2602.18418