Orbitally resolved single-photon emission from an individual atomic vacancy center in a semiconductor

Fuente: arXiv
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Autores principales: Singh, Gagandeep, Lyu, Xiaodan, Chong, Bi Qi, Tang, Ryan Li Yen, SK, Rejaul, Que, Yande, Shivajirao, Ranjith, Aliyar, Thasneem, Krishnan, Radha, Jia, Junxiang, Fuhrer, Michael S., Koh, Teck Seng, Gao, Weibo, Weber, Bent
Formato: Preprint
Publicado: 2026
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author Singh, Gagandeep
Lyu, Xiaodan
Chong, Bi Qi
Tang, Ryan Li Yen
SK, Rejaul
Que, Yande
Shivajirao, Ranjith
Aliyar, Thasneem
Krishnan, Radha
Jia, Junxiang
Fuhrer, Michael S.
Koh, Teck Seng
Gao, Weibo
Weber, Bent
author_facet Singh, Gagandeep
Lyu, Xiaodan
Chong, Bi Qi
Tang, Ryan Li Yen
SK, Rejaul
Que, Yande
Shivajirao, Ranjith
Aliyar, Thasneem
Krishnan, Radha
Jia, Junxiang
Fuhrer, Michael S.
Koh, Teck Seng
Gao, Weibo
Weber, Bent
contents Atomically confined spins are emerging as active components in quantum optoelectronic devices such as quantum bits and sensors. However, interrogating single spins at atomic length-scales remains a sizeable challenge, limited by diffraction in conventional optics. Here we show that the highly-local excitation provided by injecting energetic charge carriers from the atomically sharp probe of a scanning tunneling microscope can trigger single-photon emission from individual atomic vacancy centers in a layered semiconductor. With an effective spatial resolution of <1 nm, we show that the captured light closely mirrors the orbital symmetry of the bound-state wavefunction of the vacancy center while photon correlation measurements confirm single-photon emission, as reflected in clear photon anti-bunching signatures. Our results constitute an important step toward the realization of an electrically addressable single-atom quantum light source and solid-state spinphoton interface, addressed at the atomic-scale.
format Preprint
id arxiv_https___arxiv_org_abs_2602_23931
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Orbitally resolved single-photon emission from an individual atomic vacancy center in a semiconductor
Singh, Gagandeep
Lyu, Xiaodan
Chong, Bi Qi
Tang, Ryan Li Yen
SK, Rejaul
Que, Yande
Shivajirao, Ranjith
Aliyar, Thasneem
Krishnan, Radha
Jia, Junxiang
Fuhrer, Michael S.
Koh, Teck Seng
Gao, Weibo
Weber, Bent
Mesoscale and Nanoscale Physics
Optics
Quantum Physics
Atomically confined spins are emerging as active components in quantum optoelectronic devices such as quantum bits and sensors. However, interrogating single spins at atomic length-scales remains a sizeable challenge, limited by diffraction in conventional optics. Here we show that the highly-local excitation provided by injecting energetic charge carriers from the atomically sharp probe of a scanning tunneling microscope can trigger single-photon emission from individual atomic vacancy centers in a layered semiconductor. With an effective spatial resolution of <1 nm, we show that the captured light closely mirrors the orbital symmetry of the bound-state wavefunction of the vacancy center while photon correlation measurements confirm single-photon emission, as reflected in clear photon anti-bunching signatures. Our results constitute an important step toward the realization of an electrically addressable single-atom quantum light source and solid-state spinphoton interface, addressed at the atomic-scale.
title Orbitally resolved single-photon emission from an individual atomic vacancy center in a semiconductor
topic Mesoscale and Nanoscale Physics
Optics
Quantum Physics
url https://arxiv.org/abs/2602.23931