Tuning of superconducting properties with disorder in NbxSn nanocrystalline thin films

Fuente: arXiv
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Hauptverfasser: Poojary, Mahesh, Bathula, Vishwanadh, Kumar, Yash, Verma, Amar, Kadam, Ekta, Bose, Sangita
Format: Preprint
Veröffentlicht: 2026
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author Poojary, Mahesh
Bathula, Vishwanadh
Kumar, Yash
Verma, Amar
Kadam, Ekta
Bose, Sangita
author_facet Poojary, Mahesh
Bathula, Vishwanadh
Kumar, Yash
Verma, Amar
Kadam, Ekta
Bose, Sangita
contents Nanocrystalline superconducting films offer an excellent platform to explore the interplay between disorder, granularity, and dimensionality. In this work, we investigate two series of NbxSn thin films with near-stoichiometric (x =3) and slightly Sn-rich (x =2.5) compositions, deposited on Si (100) substrates via DC magnetron sputtering. Both series exhibit nanocrystalline morphology, with the Sn-rich films displaying smaller grain sizes and a more granular microstructure. A suppression of the superconducting transition temperature (Tc) with decreasing film thickness is observed in both series. Notably, a disorder-driven crossover to an insulating state emerges, occurring at a thickness of approximately 11 nm for the Sn-rich films-about twice that of the stoichiometric films. The estimated disorder parameter (kFl=0.4) in the thinnest films indicates proximity to the Anderson localization regime for these films. Magneto-transport measurements reveal a thickness-driven 3D to 2D crossover, with its onset strongly dependent on film stoichiometry. Furthermore, a pronounced suppression of superfluid stiffness is observed in the Sn-rich films, corroborating the structure-property correlations identified in this study. This work highlights the role of stoichiometry controlled disorder in tuning superconductivity in granular NbxSn thin films.
format Preprint
id arxiv_https___arxiv_org_abs_2603_00954
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Tuning of superconducting properties with disorder in NbxSn nanocrystalline thin films
Poojary, Mahesh
Bathula, Vishwanadh
Kumar, Yash
Verma, Amar
Kadam, Ekta
Bose, Sangita
Superconductivity
Mesoscale and Nanoscale Physics
Nanocrystalline superconducting films offer an excellent platform to explore the interplay between disorder, granularity, and dimensionality. In this work, we investigate two series of NbxSn thin films with near-stoichiometric (x =3) and slightly Sn-rich (x =2.5) compositions, deposited on Si (100) substrates via DC magnetron sputtering. Both series exhibit nanocrystalline morphology, with the Sn-rich films displaying smaller grain sizes and a more granular microstructure. A suppression of the superconducting transition temperature (Tc) with decreasing film thickness is observed in both series. Notably, a disorder-driven crossover to an insulating state emerges, occurring at a thickness of approximately 11 nm for the Sn-rich films-about twice that of the stoichiometric films. The estimated disorder parameter (kFl=0.4) in the thinnest films indicates proximity to the Anderson localization regime for these films. Magneto-transport measurements reveal a thickness-driven 3D to 2D crossover, with its onset strongly dependent on film stoichiometry. Furthermore, a pronounced suppression of superfluid stiffness is observed in the Sn-rich films, corroborating the structure-property correlations identified in this study. This work highlights the role of stoichiometry controlled disorder in tuning superconductivity in granular NbxSn thin films.
title Tuning of superconducting properties with disorder in NbxSn nanocrystalline thin films
topic Superconductivity
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2603.00954