Decoupling Intrinsic Molecular Efficacy from Platform Effects: An Interpretable Machine Learning Framework for Unbiased Perovskite Passivator Discovery

Fuente: arXiv
Saved in:
Bibliographic Details
Main Authors: Zhang, Jing, Li, Ziyuan, Gao, Shan, Zhu, Zhen, Wang, Jing, Duan, Xiangmei
Format: Preprint
Published: 2026
Subjects:
Online Access:
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1866912939379785728
author Zhang, Jing
Li, Ziyuan
Gao, Shan
Zhu, Zhen
Wang, Jing
Duan, Xiangmei
author_facet Zhang, Jing
Li, Ziyuan
Gao, Shan
Zhu, Zhen
Wang, Jing
Duan, Xiangmei
contents Rational design of interface passivators for perovskite solar cells is hindered by the entanglement of intrinsic molecular efficacy with extrinsic platform-dependent performance - a confounding factor that obscures true chemical advances. Here, we present a generalizable, interpretable machine learning framework that decouples these effects via an asymptotic saturation model, enabling unbiased discovery of molecules with genuine intrinsic gains. Trained on a curated dataset of 240 experimental entries, our model identifies hydrogen bond acceptor strength and electrostatic potential difference as key descriptors. Guided by these insights, we screened >121 million PubChem compounds using a hierarchical strategy integrating diversity clustering and uncertainty quantification. Five dual-functional candidates (e.g., TDZ-S, TZC-F) are identified, exhibiting superior predicted efficacy (surpassing experimental benchmarks) and high confidence. First-principles calculations confirm strong chemisorption (Eads<-1.7 eV), net electron donation, and optimized interfacial energetics. Crucially, our closed-loop "data-interpretation-screening-verification" pipeline establishes a transferable paradigm for rational materials design, extendable to other optoelectronic interfaces beyond perovskites.
format Preprint
id arxiv_https___arxiv_org_abs_2603_02717
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Decoupling Intrinsic Molecular Efficacy from Platform Effects: An Interpretable Machine Learning Framework for Unbiased Perovskite Passivator Discovery
Zhang, Jing
Li, Ziyuan
Gao, Shan
Zhu, Zhen
Wang, Jing
Duan, Xiangmei
Materials Science
Rational design of interface passivators for perovskite solar cells is hindered by the entanglement of intrinsic molecular efficacy with extrinsic platform-dependent performance - a confounding factor that obscures true chemical advances. Here, we present a generalizable, interpretable machine learning framework that decouples these effects via an asymptotic saturation model, enabling unbiased discovery of molecules with genuine intrinsic gains. Trained on a curated dataset of 240 experimental entries, our model identifies hydrogen bond acceptor strength and electrostatic potential difference as key descriptors. Guided by these insights, we screened >121 million PubChem compounds using a hierarchical strategy integrating diversity clustering and uncertainty quantification. Five dual-functional candidates (e.g., TDZ-S, TZC-F) are identified, exhibiting superior predicted efficacy (surpassing experimental benchmarks) and high confidence. First-principles calculations confirm strong chemisorption (Eads<-1.7 eV), net electron donation, and optimized interfacial energetics. Crucially, our closed-loop "data-interpretation-screening-verification" pipeline establishes a transferable paradigm for rational materials design, extendable to other optoelectronic interfaces beyond perovskites.
title Decoupling Intrinsic Molecular Efficacy from Platform Effects: An Interpretable Machine Learning Framework for Unbiased Perovskite Passivator Discovery
topic Materials Science
url https://arxiv.org/abs/2603.02717