Cubic-in-magnetization contributions to the magneto-optic Kerr effect investigated for Ni(001) and Ni(111) thin films

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Autori principali: Silber, Robin, Gaerner, Maik, Postava, Kamil, Hamrle, Jaroslav, Kuschel, Timo
Natura: Preprint
Pubblicazione: 2026
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author Silber, Robin
Gaerner, Maik
Postava, Kamil
Hamrle, Jaroslav
Kuschel, Timo
author_facet Silber, Robin
Gaerner, Maik
Postava, Kamil
Hamrle, Jaroslav
Kuschel, Timo
contents *The abstract of this article is too long to be included in the arXiv metadata; please see the paper for the full abstract.* ...In this paper, we introduce the detailed theory of cubic-in-magnetization magneto-optic Kerr effect (CMOKE) by deriving the magneto-optic tensor of third order in magnetization, denoted as $\bm{H}$, and comparing the strength of CMOKE for different crystal orientations theoretically and experimentally. In crystals with cubic symmetry, the tensor $\bm{H}$ is described by two independent parameters $H_{123}$ and $H_{125}$. Together with the linear magneto-optic tensor $\bm{K}$ and quadratic magento-optic tensor $\bm{G}$, the permittivity tensor is described up to third order in magnetization. We analytically describe equations of the MOKE including the contribution of QMOKE and CMOKE itself for (001)- and (111)-oriented cubic crystal structures. Those are compared to experimental measurements of two samples with an (001)- and (111)-oriented fcc Ni layer, respectively. Further, we use Yeh's 4$\times$4 transfer matrix calculus to simulate and describe the experimental measurements phenomenologically from the permittivity tensor up to third order in $\bm{M}$. We find that the MOKE anisotropy that stems from the magneto-optic tensor $\bm{H}$ described as $ΔH = H_{123}-3H_{125}$, is much more pronounced for the (111)-oriented cubic crystal structure, for which it manifests as three-fold in-plane angular dependencies of MOKE with longitudinal and also with transversal magnetization direction, respectively.
format Preprint
id arxiv_https___arxiv_org_abs_2603_03477
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Cubic-in-magnetization contributions to the magneto-optic Kerr effect investigated for Ni(001) and Ni(111) thin films
Silber, Robin
Gaerner, Maik
Postava, Kamil
Hamrle, Jaroslav
Kuschel, Timo
Optics
*The abstract of this article is too long to be included in the arXiv metadata; please see the paper for the full abstract.* ...In this paper, we introduce the detailed theory of cubic-in-magnetization magneto-optic Kerr effect (CMOKE) by deriving the magneto-optic tensor of third order in magnetization, denoted as $\bm{H}$, and comparing the strength of CMOKE for different crystal orientations theoretically and experimentally. In crystals with cubic symmetry, the tensor $\bm{H}$ is described by two independent parameters $H_{123}$ and $H_{125}$. Together with the linear magneto-optic tensor $\bm{K}$ and quadratic magento-optic tensor $\bm{G}$, the permittivity tensor is described up to third order in magnetization. We analytically describe equations of the MOKE including the contribution of QMOKE and CMOKE itself for (001)- and (111)-oriented cubic crystal structures. Those are compared to experimental measurements of two samples with an (001)- and (111)-oriented fcc Ni layer, respectively. Further, we use Yeh's 4$\times$4 transfer matrix calculus to simulate and describe the experimental measurements phenomenologically from the permittivity tensor up to third order in $\bm{M}$. We find that the MOKE anisotropy that stems from the magneto-optic tensor $\bm{H}$ described as $ΔH = H_{123}-3H_{125}$, is much more pronounced for the (111)-oriented cubic crystal structure, for which it manifests as three-fold in-plane angular dependencies of MOKE with longitudinal and also with transversal magnetization direction, respectively.
title Cubic-in-magnetization contributions to the magneto-optic Kerr effect investigated for Ni(001) and Ni(111) thin films
topic Optics
url https://arxiv.org/abs/2603.03477