X-ray magnetic circular dichroism evidence of intrinsic $d$-wave altermagnetism in rutile-structure NiF$_2$

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Hauptverfasser: Li, Zezhong, Sakurai, Kosuke, Chiu, Yiu-Fung, Backes, Dirk, Prabhakaran, Dharmalingam, Furo, Mizuki, Won, Choongjae, Zhang, Wenliang, Cheong, Sang-Wook, Boothroyd, Andrew, Garcia-Fernandez, Mirian, Tippireddy, Sahil, Kuneš, Jan, Agrestini, Stefano, Hariki, Atsushi, Zhou, Ke-Jin
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Veröffentlicht: 2026
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author Li, Zezhong
Sakurai, Kosuke
Chiu, Yiu-Fung
Backes, Dirk
Prabhakaran, Dharmalingam
Furo, Mizuki
Won, Choongjae
Zhang, Wenliang
Cheong, Sang-Wook
Boothroyd, Andrew
Garcia-Fernandez, Mirian
Tippireddy, Sahil
Kuneš, Jan
Agrestini, Stefano
Hariki, Atsushi
Zhou, Ke-Jin
author_facet Li, Zezhong
Sakurai, Kosuke
Chiu, Yiu-Fung
Backes, Dirk
Prabhakaran, Dharmalingam
Furo, Mizuki
Won, Choongjae
Zhang, Wenliang
Cheong, Sang-Wook
Boothroyd, Andrew
Garcia-Fernandez, Mirian
Tippireddy, Sahil
Kuneš, Jan
Agrestini, Stefano
Hariki, Atsushi
Zhou, Ke-Jin
contents We present the x-ray magnetic circular dichroism (XMCD) at the Ni $L_{2,3}$-edge as an evidence of the $d$-wave altermagnetism in rutile-structure NiF$_2$. Sizable XMCD signal is observed in excellent agreement with theoretical simulations. Owing to a considerable net magnetization due to spin canting, the XMCD spectrum consists of an altermagnetic signal as well as a non-negligible ferromagnetic contribution. We verify experimentally that the XMCD spectrum can be written as a sum of contributions from altermagnetism and weak ferromagnetism. Two experimental methods to isolate the ferromagnetic contribution are shown to yield essentially the same result. These are dependence of XMCD on applied magnetic fields below the Néel temperature and the XMCD measured in applied field above the Néel temperature. Our results demonstrate the utility of XMCD as a probe for altermagnetic materials with the coexisting weak ferromagnetism induced by the relativistic spin-orbit coupling.
format Preprint
id arxiv_https___arxiv_org_abs_2603_03694
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle X-ray magnetic circular dichroism evidence of intrinsic $d$-wave altermagnetism in rutile-structure NiF$_2$
Li, Zezhong
Sakurai, Kosuke
Chiu, Yiu-Fung
Backes, Dirk
Prabhakaran, Dharmalingam
Furo, Mizuki
Won, Choongjae
Zhang, Wenliang
Cheong, Sang-Wook
Boothroyd, Andrew
Garcia-Fernandez, Mirian
Tippireddy, Sahil
Kuneš, Jan
Agrestini, Stefano
Hariki, Atsushi
Zhou, Ke-Jin
Strongly Correlated Electrons
We present the x-ray magnetic circular dichroism (XMCD) at the Ni $L_{2,3}$-edge as an evidence of the $d$-wave altermagnetism in rutile-structure NiF$_2$. Sizable XMCD signal is observed in excellent agreement with theoretical simulations. Owing to a considerable net magnetization due to spin canting, the XMCD spectrum consists of an altermagnetic signal as well as a non-negligible ferromagnetic contribution. We verify experimentally that the XMCD spectrum can be written as a sum of contributions from altermagnetism and weak ferromagnetism. Two experimental methods to isolate the ferromagnetic contribution are shown to yield essentially the same result. These are dependence of XMCD on applied magnetic fields below the Néel temperature and the XMCD measured in applied field above the Néel temperature. Our results demonstrate the utility of XMCD as a probe for altermagnetic materials with the coexisting weak ferromagnetism induced by the relativistic spin-orbit coupling.
title X-ray magnetic circular dichroism evidence of intrinsic $d$-wave altermagnetism in rutile-structure NiF$_2$
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2603.03694