Sub-wavelength mid-infrared imaging of locally driven photocurrents using diamond campanile probes

Fuente: arXiv
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Auteurs principaux: Medapalli, Rajasekhar, Cottam, Nathan D., Agarwal, Khushboo, Dewes, Benjamin T., Dessmann, Nils, Gonzalez-Munoz, Sergio, Yan, Wenjing, Mišeikis, Vaidotas, Kafanov, Sergey, Mikhaylovskiy, Rostislav V., Jarvis, Samuel P., Coletti, Camilla, Redlich, Britta, Patanè, Amalia, Kolosov, Oleg V.
Format: Preprint
Publié: 2026
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author Medapalli, Rajasekhar
Cottam, Nathan D.
Agarwal, Khushboo
Dewes, Benjamin T.
Dessmann, Nils
Gonzalez-Munoz, Sergio
Yan, Wenjing
Mišeikis, Vaidotas
Kafanov, Sergey
Mikhaylovskiy, Rostislav V.
Jarvis, Samuel P.
Coletti, Camilla
Redlich, Britta
Patanè, Amalia
Kolosov, Oleg V.
author_facet Medapalli, Rajasekhar
Cottam, Nathan D.
Agarwal, Khushboo
Dewes, Benjamin T.
Dessmann, Nils
Gonzalez-Munoz, Sergio
Yan, Wenjing
Mišeikis, Vaidotas
Kafanov, Sergey
Mikhaylovskiy, Rostislav V.
Jarvis, Samuel P.
Coletti, Camilla
Redlich, Britta
Patanè, Amalia
Kolosov, Oleg V.
contents Precise and high efficiency concentration of mid-infrared (mid-IR) light into sub wavelength volumes is essential for probing low-energy excitations and achieving strong field enhancements, which can be hindered by absorption losses and coupling inefficiencies at long wavelengths. Here, we introduce an innovative diamond-based metal-insulator-metal campanile probe that adiabatically compresses free-space mid infrared light (10 \mum) into \approx 1 \mum domains. Integrated into a scanning photovoltage microscope, the probe enables sub-wavelength mapping of locally driven photocurrents in graphene, resolving polarization dependent and contact-sensitive responses at energies down to \approx 0.1 eV. Experiments reveal a photocurrent signal density enhancement of 10^3 and coupling efficiencies approaching 80%, in agreement with numerical simulations. Operation of the probe with quantum cascade and free electron lasers demonstrates a robust, spectrally tunable platform for high-resolution exploration of low-energy carrier dynamics in atomically thin materials, opening opportunities for mid-IR optoelectronics and quantum photonics.
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id arxiv_https___arxiv_org_abs_2603_04318
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Sub-wavelength mid-infrared imaging of locally driven photocurrents using diamond campanile probes
Medapalli, Rajasekhar
Cottam, Nathan D.
Agarwal, Khushboo
Dewes, Benjamin T.
Dessmann, Nils
Gonzalez-Munoz, Sergio
Yan, Wenjing
Mišeikis, Vaidotas
Kafanov, Sergey
Mikhaylovskiy, Rostislav V.
Jarvis, Samuel P.
Coletti, Camilla
Redlich, Britta
Patanè, Amalia
Kolosov, Oleg V.
Mesoscale and Nanoscale Physics
Instrumentation and Detectors
Optics
Precise and high efficiency concentration of mid-infrared (mid-IR) light into sub wavelength volumes is essential for probing low-energy excitations and achieving strong field enhancements, which can be hindered by absorption losses and coupling inefficiencies at long wavelengths. Here, we introduce an innovative diamond-based metal-insulator-metal campanile probe that adiabatically compresses free-space mid infrared light (10 \mum) into \approx 1 \mum domains. Integrated into a scanning photovoltage microscope, the probe enables sub-wavelength mapping of locally driven photocurrents in graphene, resolving polarization dependent and contact-sensitive responses at energies down to \approx 0.1 eV. Experiments reveal a photocurrent signal density enhancement of 10^3 and coupling efficiencies approaching 80%, in agreement with numerical simulations. Operation of the probe with quantum cascade and free electron lasers demonstrates a robust, spectrally tunable platform for high-resolution exploration of low-energy carrier dynamics in atomically thin materials, opening opportunities for mid-IR optoelectronics and quantum photonics.
title Sub-wavelength mid-infrared imaging of locally driven photocurrents using diamond campanile probes
topic Mesoscale and Nanoscale Physics
Instrumentation and Detectors
Optics
url https://arxiv.org/abs/2603.04318