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Bibliographic Details
Main Authors: Bylinkin, Andrei, Roelli, Philippe, Shetty, Naveen, Yakimova, Rositsa, Starke, Ulrich, Coletti, Camilla, Forti, Stiven, Zakharov, Alexei, Silkin, Vyacheslav M., Lara-Avila, Samuel, Hillenbrand, Rainer
Format: Preprint
Published: 2026
Subjects:
Online Access:https://arxiv.org/abs/2603.05030
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Table of Contents:
  • Atomically thin materials exhibit electronic and optical properties distinct from their three-dimensional counterparts. For metals, particularly gold, monolayer studies remain largely unexplored due to fabrication and characterisation challenges. Here we report the first optical study of a stable quasi-freestanding gold monolayer formed by Au intercalation between graphene and SiC. Mid-infrared nanoimaging reveals plasmon-polaritons with wavelengths nearly an order of magnitude shorter than free-space light. Analysis of their dispersion using a Drude model yields a relaxation time of $τ= 18\,$fs, comparable to bulk gold, and a Drude weight of $D = 1.3\,$mS$\cdot$eV, nearly twice the bulk expectation. These results establish monolayer gold as a two-dimensional metal, opening opportunities for nanoscale photonics, plasmonics and ultra-thin electronics.