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Bibliographic Details
Main Authors: Mukherjee, Sounak, Li, Anran, Eberle, Johannes, Karg, Sean, Zhang, Zi-Huai, Feldman, Mayer M., Chen, Yilin, Turiansky, Mark E., Wang, Mengen, Limbu, Yogendra, Puel, Tharnier O., Shi, Yueguang, Markham, Matthew L., Patel, Rajesh L., Gumann, Patryk, Flatte, Michael E., Van de Walle, Chris G., Lyon, Stephen A., de Leon, Nathalie P.
Format: Preprint
Published: 2026
Subjects:
Online Access:https://arxiv.org/abs/2603.07265
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Table of Contents:
  • Spin defects in diamond are promising platforms for quantum sensing. The longest electron spin relaxation times ($T_1$) at room temperature for solid-state defects are observed in nitrogen vacancy centers in diamond, which can reach 6.67 ms, and substitutional nitrogen ("P1 centers") in diamond, which exhibit a $T_1$ of 2 ms. No other solid-state defect has exhibited millisecond-scale spin relaxation times at room temperature thus far. Here, we characterize the spin properties of the WAR5 defect in diamond with pulsed electron spin resonance. The observed $T_1$ is one of the longest for solid-state spin defects: 0.97(27) ms at room temperature and 14.38(19) min at 4 K. The observed coherence time ($T_2$) is 246(7) $μ$s, which can be extended to 6.49(34) ms at 4 K with dynamical decoupling. Furthermore, we demonstrate optical spin polarization with a range of wavelengths from 405 nm to 500 nm and propose potential zero-phonon line candidates.