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Main Authors: Watanabe, Shinji, Iwasaki, Tatsuya
Format: Preprint
Published: 2026
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Online Access:https://arxiv.org/abs/2603.10716
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author Watanabe, Shinji
Iwasaki, Tatsuya
author_facet Watanabe, Shinji
Iwasaki, Tatsuya
contents Ground-state properties of rare-earth based 1/1 periodic approximants of icosahedral quasicrystal are clarified theoretically on the basis of an effective model for magnetism taking into account uniaxial anisotropy arising from crystalline electric field. By performing numerically-exact calculation on the 1/1 approximant crystal with a lattice constant $a$=14.725 Å, we have determined the ground-state phase diagram for ferromagnetic interactions. The result shows that eight kinds of noncollinear and noncoplanar magnetic structures are stabilized, whose magnetic space groups are identified as $I_{\rm P}m'\bar{3}'$, $C2'/m'$ and $R\bar{3}$. We have clarified the degeneracy of each ground state, which is expected to be reflected in the numbers of the domains. By analyzing each state, the magnetic as well as topological properties are revealed. Our results are shown to explain the measured magnetic structures in the 1/1 approximants and the effective model is discussed to be useful for understanding the magnetic structures and their topological properties in broad range of rare-earth based 1/1 approximants.
format Preprint
id arxiv_https___arxiv_org_abs_2603_10716
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Non-Collinear and Non-Coplanar Magnetic Orders in 1/1 Periodic Approximant to the Icosahedral Quasicrystal
Watanabe, Shinji
Iwasaki, Tatsuya
Strongly Correlated Electrons
Materials Science
Ground-state properties of rare-earth based 1/1 periodic approximants of icosahedral quasicrystal are clarified theoretically on the basis of an effective model for magnetism taking into account uniaxial anisotropy arising from crystalline electric field. By performing numerically-exact calculation on the 1/1 approximant crystal with a lattice constant $a$=14.725 Å, we have determined the ground-state phase diagram for ferromagnetic interactions. The result shows that eight kinds of noncollinear and noncoplanar magnetic structures are stabilized, whose magnetic space groups are identified as $I_{\rm P}m'\bar{3}'$, $C2'/m'$ and $R\bar{3}$. We have clarified the degeneracy of each ground state, which is expected to be reflected in the numbers of the domains. By analyzing each state, the magnetic as well as topological properties are revealed. Our results are shown to explain the measured magnetic structures in the 1/1 approximants and the effective model is discussed to be useful for understanding the magnetic structures and their topological properties in broad range of rare-earth based 1/1 approximants.
title Non-Collinear and Non-Coplanar Magnetic Orders in 1/1 Periodic Approximant to the Icosahedral Quasicrystal
topic Strongly Correlated Electrons
Materials Science
url https://arxiv.org/abs/2603.10716