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Main Authors: Wang, Ke, Wang, Maosen, Wei, Wei, Hao, Bo, Liu, Mengqin, Xiang, Qiaochao, Zhou, Xin, Hou, Qiang, Sun, Yue, Zhu, Zengwei, Li, Sheng, Nie, Yuefeng, Shi, Zhixiang
Format: Preprint
Published: 2026
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Online Access:https://arxiv.org/abs/2603.10717
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author Wang, Ke
Wang, Maosen
Wei, Wei
Hao, Bo
Liu, Mengqin
Xiang, Qiaochao
Zhou, Xin
Hou, Qiang
Sun, Yue
Zhu, Zengwei
Li, Sheng
Nie, Yuefeng
Shi, Zhixiang
author_facet Wang, Ke
Wang, Maosen
Wei, Wei
Hao, Bo
Liu, Mengqin
Xiang, Qiaochao
Zhou, Xin
Hou, Qiang
Sun, Yue
Zhu, Zengwei
Li, Sheng
Nie, Yuefeng
Shi, Zhixiang
contents We investigate the upper critical field and superconducting anisotropy of epitaxial La2.82Sr0.18Ni2O7 thin films, which show a sharp superconducting transition at Tc=31.6 K. Near Tc, superconductivity exhibits thickness-limited two-dimensional characteristics. Upon cooling, the out-of-plane coherence length decreases below the sample thickness of 6 nm, corresponding to a 3-unit-cell film, indicating a crossover to intrinsic three-dimensional bulk superconductivity. High-field transport measurements reveal large upper critical fields with a small anisotropy ratio gama~1.34, comparable to bulk Ruddlesden-Popper nickelates. At low temperatures, the in-plane (ab) upper critical field Hc2(ab) is strongly suppressed by spin-paramagnetic pair breaking and approaches the Pauli limit (Hc2(Pauli)=58 T), while Hc2(c) remains largely unaffected. This anisotropic Pauli limitation accounts for the reduced upper critical field anisotropy and supports the conclusion that superconductivity in these films is fundamentally three-dimensional bulk like. Our results highlight the essential role of spin-paramagnetic effects in shaping the high-field superconducting phase diagram of Ruddlesden-Popper nickelates.
format Preprint
id arxiv_https___arxiv_org_abs_2603_10717
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Pauli-limited upper critical field and anisotropic depairing effect of La2.82Sr0.18Ni2O7 superconducting thin film
Wang, Ke
Wang, Maosen
Wei, Wei
Hao, Bo
Liu, Mengqin
Xiang, Qiaochao
Zhou, Xin
Hou, Qiang
Sun, Yue
Zhu, Zengwei
Li, Sheng
Nie, Yuefeng
Shi, Zhixiang
Superconductivity
We investigate the upper critical field and superconducting anisotropy of epitaxial La2.82Sr0.18Ni2O7 thin films, which show a sharp superconducting transition at Tc=31.6 K. Near Tc, superconductivity exhibits thickness-limited two-dimensional characteristics. Upon cooling, the out-of-plane coherence length decreases below the sample thickness of 6 nm, corresponding to a 3-unit-cell film, indicating a crossover to intrinsic three-dimensional bulk superconductivity. High-field transport measurements reveal large upper critical fields with a small anisotropy ratio gama~1.34, comparable to bulk Ruddlesden-Popper nickelates. At low temperatures, the in-plane (ab) upper critical field Hc2(ab) is strongly suppressed by spin-paramagnetic pair breaking and approaches the Pauli limit (Hc2(Pauli)=58 T), while Hc2(c) remains largely unaffected. This anisotropic Pauli limitation accounts for the reduced upper critical field anisotropy and supports the conclusion that superconductivity in these films is fundamentally three-dimensional bulk like. Our results highlight the essential role of spin-paramagnetic effects in shaping the high-field superconducting phase diagram of Ruddlesden-Popper nickelates.
title Pauli-limited upper critical field and anisotropic depairing effect of La2.82Sr0.18Ni2O7 superconducting thin film
topic Superconductivity
url https://arxiv.org/abs/2603.10717