Dissipative self-assembly of colloidal suspensions

Fuente: arXiv
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Autores principales: Conradt, Jason, Furst, Eric M.
Formato: Preprint
Publicado: 2026
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author Conradt, Jason
Furst, Eric M.
author_facet Conradt, Jason
Furst, Eric M.
contents Suspensions of paramagnetic colloids exhibit kinetic arrest in strong magnetic fields. Through a dissipative process of toggling the field on and off, suspensions self-assemble into dense and dynamic steady-state phases. Based on the domain elongation, alpha- and contour-shapes, and degree of phase separation, we construct a phase diagram using a k-means clustering analysis. We identify six characteristic structural regimes: a structureless phase, an arrested structure, sheets, ribbons, a spiky phase, and a transient fluid-fluid regime. We further report the distribution and alignment of domains and the generality of the results. We model self-assembled domain shapes using an equilibrium mean-field magnetostatic energy calculation, which predicts the surprising emergence of highly-anisotropic structures driven by the sample's confinement.
format Preprint
id arxiv_https___arxiv_org_abs_2603_14637
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Dissipative self-assembly of colloidal suspensions
Conradt, Jason
Furst, Eric M.
Soft Condensed Matter
Suspensions of paramagnetic colloids exhibit kinetic arrest in strong magnetic fields. Through a dissipative process of toggling the field on and off, suspensions self-assemble into dense and dynamic steady-state phases. Based on the domain elongation, alpha- and contour-shapes, and degree of phase separation, we construct a phase diagram using a k-means clustering analysis. We identify six characteristic structural regimes: a structureless phase, an arrested structure, sheets, ribbons, a spiky phase, and a transient fluid-fluid regime. We further report the distribution and alignment of domains and the generality of the results. We model self-assembled domain shapes using an equilibrium mean-field magnetostatic energy calculation, which predicts the surprising emergence of highly-anisotropic structures driven by the sample's confinement.
title Dissipative self-assembly of colloidal suspensions
topic Soft Condensed Matter
url https://arxiv.org/abs/2603.14637