Quantifying quasiparticle chirality in a chiral topological semimetal

Fuente: arXiv
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Autores principales: Wang, Jiaju, Sánchez-Barriga, Jaime, Kumar, Amit, Pardo-Almanza, Markel, Cardenas-Gamboa, Jorge, Robredo, Iñigo, Shekhar, Chandra, Geng, Daiyu, McFarlane, Emily C., Trautmann, Martin, Della Valle, Enrico, Hoesch, Moritz, Huang, Meng-Jie, Buck, Jens, Strocov, Vladimir N., Johansson, Annika, Parkin, Stuart S. P., Felser, Claudia, Vergniory, Maia G., Schröter, Niels B. M.
Formato: Preprint
Publicado: 2026
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author Wang, Jiaju
Sánchez-Barriga, Jaime
Kumar, Amit
Pardo-Almanza, Markel
Cardenas-Gamboa, Jorge
Robredo, Iñigo
Shekhar, Chandra
Geng, Daiyu
McFarlane, Emily C.
Trautmann, Martin
Della Valle, Enrico
Hoesch, Moritz
Huang, Meng-Jie
Buck, Jens
Strocov, Vladimir N.
Johansson, Annika
Parkin, Stuart S. P.
Felser, Claudia
Vergniory, Maia G.
Schröter, Niels B. M.
author_facet Wang, Jiaju
Sánchez-Barriga, Jaime
Kumar, Amit
Pardo-Almanza, Markel
Cardenas-Gamboa, Jorge
Robredo, Iñigo
Shekhar, Chandra
Geng, Daiyu
McFarlane, Emily C.
Trautmann, Martin
Della Valle, Enrico
Hoesch, Moritz
Huang, Meng-Jie
Buck, Jens
Strocov, Vladimir N.
Johansson, Annika
Parkin, Stuart S. P.
Felser, Claudia
Vergniory, Maia G.
Schröter, Niels B. M.
contents Recently, the projection of the electron's spin on its crystal momentum has been proposed as a metric to quantify electronic chirality of Bloch states in crystals, which is expected to affect a wide range of physical properties, such as magnetoelectric and optical responses. However, a direct experimental quantification of this chirality metric over an entire iso-energy surface has remained elusive. Here, we have used spin- and angle-resolved photoemission spectroscopy to directly probe the electronic chirality by measuring the bulk spin texture of Kramers-Weyl and Weyl cones in RhSi, a chiral topological semimetal with strong spin-orbit coupling (SOC). After quantifying the SOC splitting of Weyl cones, we determine their spin direction along different azimuthal angles to extract energy dependent the deviations (up to ~40°) from perfect parallel spin-momentum locking. From these deviations we define an energy-dependent normalized electron chirality density (NECD), a directly accessible metric of bulk electronic chirality. In RhSi, the NECD decreases from 1 at the Kramers-Weyl point to ~0.8 at ~200 meV below it. Finally, we show that this experimentally grounded NECD provides predictive power for magneto-optical and transport responses of chiral materials, exemplified by the longitudinal Edelstein effect.
format Preprint
id arxiv_https___arxiv_org_abs_2603_14640
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Quantifying quasiparticle chirality in a chiral topological semimetal
Wang, Jiaju
Sánchez-Barriga, Jaime
Kumar, Amit
Pardo-Almanza, Markel
Cardenas-Gamboa, Jorge
Robredo, Iñigo
Shekhar, Chandra
Geng, Daiyu
McFarlane, Emily C.
Trautmann, Martin
Della Valle, Enrico
Hoesch, Moritz
Huang, Meng-Jie
Buck, Jens
Strocov, Vladimir N.
Johansson, Annika
Parkin, Stuart S. P.
Felser, Claudia
Vergniory, Maia G.
Schröter, Niels B. M.
Mesoscale and Nanoscale Physics
Other Condensed Matter
Recently, the projection of the electron's spin on its crystal momentum has been proposed as a metric to quantify electronic chirality of Bloch states in crystals, which is expected to affect a wide range of physical properties, such as magnetoelectric and optical responses. However, a direct experimental quantification of this chirality metric over an entire iso-energy surface has remained elusive. Here, we have used spin- and angle-resolved photoemission spectroscopy to directly probe the electronic chirality by measuring the bulk spin texture of Kramers-Weyl and Weyl cones in RhSi, a chiral topological semimetal with strong spin-orbit coupling (SOC). After quantifying the SOC splitting of Weyl cones, we determine their spin direction along different azimuthal angles to extract energy dependent the deviations (up to ~40°) from perfect parallel spin-momentum locking. From these deviations we define an energy-dependent normalized electron chirality density (NECD), a directly accessible metric of bulk electronic chirality. In RhSi, the NECD decreases from 1 at the Kramers-Weyl point to ~0.8 at ~200 meV below it. Finally, we show that this experimentally grounded NECD provides predictive power for magneto-optical and transport responses of chiral materials, exemplified by the longitudinal Edelstein effect.
title Quantifying quasiparticle chirality in a chiral topological semimetal
topic Mesoscale and Nanoscale Physics
Other Condensed Matter
url https://arxiv.org/abs/2603.14640