Acrylamide Conformers: A Revision of Published Density Functional Theory Studies

Fuente: arXiv
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Main Authors: Scott, William, Blaisten-Barojas, Estela
Format: Preprint
Published: 2026
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author Scott, William
Blaisten-Barojas, Estela
author_facet Scott, William
Blaisten-Barojas, Estela
contents Acrylamide, with PubChem identifier CID=6579 is broadcasted to have four stable conformers contrasting with several journal publications characterizing only two or three. In this revision summary the discrepancy is clarified. Through very high precision density functional theory (DFT) calculations, three stable conformers and the three transition state barriers existing between them are verified to exist and validated with our own DFT calculations The most stable conformer is a planar molecular structure termed "sys" or "trans" in the literature. Meanwhile, a less stable structure termed "skew" pertains to two 3-dimensional structures that are energy-degenerate, but differ in their structure for being mirrored images of each other. Vibrational spectra, partial atomic charges, Cartesian coordinates, and Intrinsic Reaction Coordinate paths are summarized and recalculated with DFT at the $ω$B97XD/Def2TZVPP level for the three stable acrylamide isomers: the sys/trans lowest in energy structure, and the two skew mirrored structures.
format Preprint
id arxiv_https___arxiv_org_abs_2603_14675
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Acrylamide Conformers: A Revision of Published Density Functional Theory Studies
Scott, William
Blaisten-Barojas, Estela
Materials Science
Chemical Physics
Acrylamide, with PubChem identifier CID=6579 is broadcasted to have four stable conformers contrasting with several journal publications characterizing only two or three. In this revision summary the discrepancy is clarified. Through very high precision density functional theory (DFT) calculations, three stable conformers and the three transition state barriers existing between them are verified to exist and validated with our own DFT calculations The most stable conformer is a planar molecular structure termed "sys" or "trans" in the literature. Meanwhile, a less stable structure termed "skew" pertains to two 3-dimensional structures that are energy-degenerate, but differ in their structure for being mirrored images of each other. Vibrational spectra, partial atomic charges, Cartesian coordinates, and Intrinsic Reaction Coordinate paths are summarized and recalculated with DFT at the $ω$B97XD/Def2TZVPP level for the three stable acrylamide isomers: the sys/trans lowest in energy structure, and the two skew mirrored structures.
title Acrylamide Conformers: A Revision of Published Density Functional Theory Studies
topic Materials Science
Chemical Physics
url https://arxiv.org/abs/2603.14675