Stoichiometric FeTe is a Superconductor

Fuente: arXiv
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Autori principali: Yan, Zi-Jie, Wang, Zihao, Xia, Bing, Paolini, Stephen, Chan, Ying-Ting, Dihingia, Nikalabh, Rong, Hongtao, Xiao, Pu, Halanayake, Kalana D., Song, Jiatao, Gowda, Veer, Hickey, Danielle Reifsnyder, Wu, Weida, Yu, Jiabin, Hirschfeld, Peter J., Chang, Cui-Zu
Natura: Preprint
Pubblicazione: 2026
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author Yan, Zi-Jie
Wang, Zihao
Xia, Bing
Paolini, Stephen
Chan, Ying-Ting
Dihingia, Nikalabh
Rong, Hongtao
Xiao, Pu
Halanayake, Kalana D.
Song, Jiatao
Gowda, Veer
Hickey, Danielle Reifsnyder
Wu, Weida
Yu, Jiabin
Hirschfeld, Peter J.
Chang, Cui-Zu
author_facet Yan, Zi-Jie
Wang, Zihao
Xia, Bing
Paolini, Stephen
Chan, Ying-Ting
Dihingia, Nikalabh
Rong, Hongtao
Xiao, Pu
Halanayake, Kalana D.
Song, Jiatao
Gowda, Veer
Hickey, Danielle Reifsnyder
Wu, Weida
Yu, Jiabin
Hirschfeld, Peter J.
Chang, Cui-Zu
contents Iron-based superconductors are a fascinating family of materials in which multiple electronic bands and strong antiferromagnetic (AFM) correlations are key ingredients for competing ground states, including antiferromagnetism, electronic nematicity, and unconventional superconductivity. FeTe, unlike its superconducting isostructural counterpart FeSe, has long been regarded as an AFM metal sans superconductivity. In this work, we employ molecular beam epitaxy to grow FeTe films and perform post-growth annealing under a Te flux. By performing spin-polarized scanning tunneling microscopy and spectroscopy, we demonstrate that the AFM order in as-grown FeTe films is induced by interstitial Fe atoms that disrupt the ideal 1:1 stoichiometry. Remarkably, the removal of these interstitial Fe atoms through Te annealing yields stoichiometric FeTe films that show no AFM order and instead exhibit robust superconductivity with a critical temperature of ~13.5K. This superconducting state is further confirmed by the observation of Cooper pair tunneling, zero electrical resistance, and the Meissner effect. Therefore, our results demonstrate that stoichiometric FeTe is inherently a superconductor, overturning a long-held view that it is an AFM metal. This work clarifies the origin of superconductivity in FeTe-based heterostructures and demonstrates the importance of stoichiometry control in understanding the competition between AFM and superconductivity in iron-based superconductors.
format Preprint
id arxiv_https___arxiv_org_abs_2603_16115
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Stoichiometric FeTe is a Superconductor
Yan, Zi-Jie
Wang, Zihao
Xia, Bing
Paolini, Stephen
Chan, Ying-Ting
Dihingia, Nikalabh
Rong, Hongtao
Xiao, Pu
Halanayake, Kalana D.
Song, Jiatao
Gowda, Veer
Hickey, Danielle Reifsnyder
Wu, Weida
Yu, Jiabin
Hirschfeld, Peter J.
Chang, Cui-Zu
Superconductivity
Mesoscale and Nanoscale Physics
Materials Science
Iron-based superconductors are a fascinating family of materials in which multiple electronic bands and strong antiferromagnetic (AFM) correlations are key ingredients for competing ground states, including antiferromagnetism, electronic nematicity, and unconventional superconductivity. FeTe, unlike its superconducting isostructural counterpart FeSe, has long been regarded as an AFM metal sans superconductivity. In this work, we employ molecular beam epitaxy to grow FeTe films and perform post-growth annealing under a Te flux. By performing spin-polarized scanning tunneling microscopy and spectroscopy, we demonstrate that the AFM order in as-grown FeTe films is induced by interstitial Fe atoms that disrupt the ideal 1:1 stoichiometry. Remarkably, the removal of these interstitial Fe atoms through Te annealing yields stoichiometric FeTe films that show no AFM order and instead exhibit robust superconductivity with a critical temperature of ~13.5K. This superconducting state is further confirmed by the observation of Cooper pair tunneling, zero electrical resistance, and the Meissner effect. Therefore, our results demonstrate that stoichiometric FeTe is inherently a superconductor, overturning a long-held view that it is an AFM metal. This work clarifies the origin of superconductivity in FeTe-based heterostructures and demonstrates the importance of stoichiometry control in understanding the competition between AFM and superconductivity in iron-based superconductors.
title Stoichiometric FeTe is a Superconductor
topic Superconductivity
Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2603.16115