Comment on "Efficient implementation of the superposition of atomic potentials initial guess for electronic structure calculations in Gaussian basis sets"

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Main Authors: Surjuse, Kshitijkumar A., Deng, Zhihao, Asadchev, Andrey, Valeev, Edward F.
Format: Preprint
Published: 2026
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author Surjuse, Kshitijkumar A.
Deng, Zhihao
Asadchev, Andrey
Valeev, Edward F.
author_facet Surjuse, Kshitijkumar A.
Deng, Zhihao
Asadchev, Andrey
Valeev, Edward F.
contents In J. Chem. Phys. 152, 144105 (2020) Lehtola et al introduced the efficient Gaussian-basis representation of Superposition of Atomic Potentials (SAP) which "can be easily implemented in any Gaussian-basis quantum chemistry code in terms of two-electron integrals". Here we demonstrate that it is possible to evaluate Gaussian AO representation of SAP by nearly trivial modification of one-electron nuclear attraction integrals.
format Preprint
id arxiv_https___arxiv_org_abs_2603_16989
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Comment on "Efficient implementation of the superposition of atomic potentials initial guess for electronic structure calculations in Gaussian basis sets"
Surjuse, Kshitijkumar A.
Deng, Zhihao
Asadchev, Andrey
Valeev, Edward F.
Chemical Physics
In J. Chem. Phys. 152, 144105 (2020) Lehtola et al introduced the efficient Gaussian-basis representation of Superposition of Atomic Potentials (SAP) which "can be easily implemented in any Gaussian-basis quantum chemistry code in terms of two-electron integrals". Here we demonstrate that it is possible to evaluate Gaussian AO representation of SAP by nearly trivial modification of one-electron nuclear attraction integrals.
title Comment on "Efficient implementation of the superposition of atomic potentials initial guess for electronic structure calculations in Gaussian basis sets"
topic Chemical Physics
url https://arxiv.org/abs/2603.16989