Diffusion-based Probabilistic Air Quality Forecasting with Mechanistic Insight

Fuente: arXiv
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Auteurs principaux: Ding, Ao, Zhang, Aoxing, Fu, Tzung-May, Huang, Yuanlong, Chen, Qianjie, Chen, Yuyang, Mo, Jiajia, Tao, Wei, Cheng, Wai-Chi, Zhu, Lei, Yang, Xin, Brasseur, Guy
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Publié: 2026
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author Ding, Ao
Zhang, Aoxing
Fu, Tzung-May
Huang, Yuanlong
Chen, Qianjie
Chen, Yuyang
Mo, Jiajia
Tao, Wei
Cheng, Wai-Chi
Zhu, Lei
Yang, Xin
Brasseur, Guy
author_facet Ding, Ao
Zhang, Aoxing
Fu, Tzung-May
Huang, Yuanlong
Chen, Qianjie
Chen, Yuyang
Mo, Jiajia
Tao, Wei
Cheng, Wai-Chi
Zhu, Lei
Yang, Xin
Brasseur, Guy
contents Current operational air quality forecasts are computationally expensive, sensitive to errors in physics and emissions, and often neglect weather-related uncertainty. To address these limitations, we present AirFusion, a hybrid, diffusion-based framework that synergistically integrates knowledge from chemical transport models with real-world observational constraints to enable accurate and efficient probabilistic regional air quality prediction. We apply AirFusion to generate operational 6-day, 30-member ensemble forecasts of surface ozone across China, initialized with observations and driven by ensemble weather forecasts. AirFusion outperforms existing operational benchmarks, achieving substantially lower forecast errors against surface measurements, while also providing ensemble-based diagnostics that explicitly quantify the impacts of weather uncertainty on air quality predictability. Moreover, AirFusion can rapidly adapt to evolving emissions through fine-tuning with only one month of recent observations. These attributes establish AirFusion as a powerful and extensible framework for next-generation probabilistic air quality forecasting, with clear potential for application to other pollutants and regions.
format Preprint
id arxiv_https___arxiv_org_abs_2603_21131
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Diffusion-based Probabilistic Air Quality Forecasting with Mechanistic Insight
Ding, Ao
Zhang, Aoxing
Fu, Tzung-May
Huang, Yuanlong
Chen, Qianjie
Chen, Yuyang
Mo, Jiajia
Tao, Wei
Cheng, Wai-Chi
Zhu, Lei
Yang, Xin
Brasseur, Guy
Atmospheric and Oceanic Physics
Current operational air quality forecasts are computationally expensive, sensitive to errors in physics and emissions, and often neglect weather-related uncertainty. To address these limitations, we present AirFusion, a hybrid, diffusion-based framework that synergistically integrates knowledge from chemical transport models with real-world observational constraints to enable accurate and efficient probabilistic regional air quality prediction. We apply AirFusion to generate operational 6-day, 30-member ensemble forecasts of surface ozone across China, initialized with observations and driven by ensemble weather forecasts. AirFusion outperforms existing operational benchmarks, achieving substantially lower forecast errors against surface measurements, while also providing ensemble-based diagnostics that explicitly quantify the impacts of weather uncertainty on air quality predictability. Moreover, AirFusion can rapidly adapt to evolving emissions through fine-tuning with only one month of recent observations. These attributes establish AirFusion as a powerful and extensible framework for next-generation probabilistic air quality forecasting, with clear potential for application to other pollutants and regions.
title Diffusion-based Probabilistic Air Quality Forecasting with Mechanistic Insight
topic Atmospheric and Oceanic Physics
url https://arxiv.org/abs/2603.21131