Efficient photo-Nernst terahertz emission in single heavy-metal films

Fuente: arXiv
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Autori principali: Wang, Lei, Song, Linxuan, Chia, Elbert E. M., Sun, Peijie, Luo, Jianlin, Chen, Rongyan, Lau, Yong-Chang, Wang, Xinbo
Natura: Preprint
Pubblicazione: 2026
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author Wang, Lei
Song, Linxuan
Chia, Elbert E. M.
Sun, Peijie
Luo, Jianlin
Chen, Rongyan
Lau, Yong-Chang
Wang, Xinbo
author_facet Wang, Lei
Song, Linxuan
Chia, Elbert E. M.
Sun, Peijie
Luo, Jianlin
Chen, Rongyan
Lau, Yong-Chang
Wang, Xinbo
contents State-of-the-art metallic terahertz (THz) emitters rely predominantly on spintronic heterostructures, where heavy metals serve as passive spin-to-charge converters. Here, we demonstrate efficient THz radiation from standalone Pt nanofilms at cryogenic temperatures and under external magnetic fields. The governing mechanism is identified as the ultrafast photo-Nernst effect, wherein a transient thermal gradient drives a transverse charge current. The THz emission polarity is directly dictated by the sign of the Nernst coefficient, as verified by the phase reversal observed between Pt and W or Ta. Remarkably, both thickness scaling and alloying-induced suppression of thermal conductivity independently amplify the single-layer emission to levels comparable with benchmark spintronic bilayers. These findings redefine the established role of heavy metals from passive spin-sinks to active THz emitters, uncovering a universal emission paradigm applicable across diverse spintronic and quantum materials.
format Preprint
id arxiv_https___arxiv_org_abs_2603_21924
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Efficient photo-Nernst terahertz emission in single heavy-metal films
Wang, Lei
Song, Linxuan
Chia, Elbert E. M.
Sun, Peijie
Luo, Jianlin
Chen, Rongyan
Lau, Yong-Chang
Wang, Xinbo
Mesoscale and Nanoscale Physics
Optics
State-of-the-art metallic terahertz (THz) emitters rely predominantly on spintronic heterostructures, where heavy metals serve as passive spin-to-charge converters. Here, we demonstrate efficient THz radiation from standalone Pt nanofilms at cryogenic temperatures and under external magnetic fields. The governing mechanism is identified as the ultrafast photo-Nernst effect, wherein a transient thermal gradient drives a transverse charge current. The THz emission polarity is directly dictated by the sign of the Nernst coefficient, as verified by the phase reversal observed between Pt and W or Ta. Remarkably, both thickness scaling and alloying-induced suppression of thermal conductivity independently amplify the single-layer emission to levels comparable with benchmark spintronic bilayers. These findings redefine the established role of heavy metals from passive spin-sinks to active THz emitters, uncovering a universal emission paradigm applicable across diverse spintronic and quantum materials.
title Efficient photo-Nernst terahertz emission in single heavy-metal films
topic Mesoscale and Nanoscale Physics
Optics
url https://arxiv.org/abs/2603.21924