Anisotropic light-electron-phonon coupling and ultrafast carrier separation in ferroelectric BaTiO$_3$

Fuente: arXiv
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Autori principali: Swain, Atal Bihari, Kale, Somnath, Soni, Rohit, Baum, Peter
Natura: Preprint
Pubblicazione: 2026
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author Swain, Atal Bihari
Kale, Somnath
Soni, Rohit
Baum, Peter
author_facet Swain, Atal Bihari
Kale, Somnath
Soni, Rohit
Baum, Peter
contents Ferroelectric materials with built-in electric fields are useful for ultrafast electronics and solar cells. Using ultrafast electron diffraction, we here report that ferroelectric BaTiO$_3$ reacts to light with a polarization-sensitive electron-phonon coupling. Excited electrons relax faster into phonons and temperature when the optical electric field aligns to the ferroelectric polarization. Also, ultrafast electron electrometry visualizes the motion of photo-excited electron-hole pairs in presence of the ferroelectric field.
format Preprint
id arxiv_https___arxiv_org_abs_2603_25521
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Anisotropic light-electron-phonon coupling and ultrafast carrier separation in ferroelectric BaTiO$_3$
Swain, Atal Bihari
Kale, Somnath
Soni, Rohit
Baum, Peter
Materials Science
Other Condensed Matter
Ferroelectric materials with built-in electric fields are useful for ultrafast electronics and solar cells. Using ultrafast electron diffraction, we here report that ferroelectric BaTiO$_3$ reacts to light with a polarization-sensitive electron-phonon coupling. Excited electrons relax faster into phonons and temperature when the optical electric field aligns to the ferroelectric polarization. Also, ultrafast electron electrometry visualizes the motion of photo-excited electron-hole pairs in presence of the ferroelectric field.
title Anisotropic light-electron-phonon coupling and ultrafast carrier separation in ferroelectric BaTiO$_3$
topic Materials Science
Other Condensed Matter
url https://arxiv.org/abs/2603.25521