Antiferromagnetic stripe phase and large-gap insulating ground state of the correlated $\sqrt{3}\times\sqrt{3}$~R30$^{\circ}$-Sn/Si(111) single atomic layer

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Main Authors: Torkzadeh, Mohammadmehdi, Iannetti, Mattia, Lizée, Mathieu, Thakur, Amitayhush, Hervé, Maris, Debontridder, Francois, David, Pascal, Casula, Michele, Profeta, Gianni, Cren, Tristan, Calandra, Matteo, Tresca, Cesare, Brun, Christophe
Format: Preprint
Published: 2026
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author Torkzadeh, Mohammadmehdi
Iannetti, Mattia
Lizée, Mathieu
Thakur, Amitayhush
Hervé, Maris
Debontridder, Francois
David, Pascal
Casula, Michele
Profeta, Gianni
Cren, Tristan
Calandra, Matteo
Tresca, Cesare
Brun, Christophe
author_facet Torkzadeh, Mohammadmehdi
Iannetti, Mattia
Lizée, Mathieu
Thakur, Amitayhush
Hervé, Maris
Debontridder, Francois
David, Pascal
Casula, Michele
Profeta, Gianni
Cren, Tristan
Calandra, Matteo
Tresca, Cesare
Brun, Christophe
contents The one-third monolayer Sn layer on Si(111) has long been considered a benchmark system for exploring two-dimensional Mott physics, owing to its narrow bandwidth and sizable on-site Coulomb repulsion. Previous experiments suggested the emergence of a low-temperature Mott insulating phase with an energy gap of only a few tens of meV, while theory predicted a possible antiferromagnetic ordering that remained experimentally elusive. Here, by combining low-temperature scanning tunneling microscopy/spectroscopy with first-principles calculations, we reveal that the $\sqrt{3}\times\sqrt{3}$~R30$^{\circ}$-Sn/Si(111) surface undergoes a transition below 30K into a robust insulating state characterized by a remarkably large gap of about 440 $\pm$ 120 meV at 4K, five to ten times larger than previously reported. Quasiparticle interference imaging uncovers a well-defined $2\sqrt{3}\times\sqrt{3}$~R30$^{\circ}$-Sn/Si(111) superstructure, providing direct evidence for a two-dimensional stripe-like antiferromagnetic order. Ab initio calculations reveal that the silicon substrate stabilizes this phase through strong nonlocal tin-tin interactions, highlighting the decisive role of substrate-driven correlations in the $\sqrt{3}\times\sqrt{3}$~R30$^{\circ}$-Sn/Si(111) system.
format Preprint
id arxiv_https___arxiv_org_abs_2603_26304
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Antiferromagnetic stripe phase and large-gap insulating ground state of the correlated $\sqrt{3}\times\sqrt{3}$~R30$^{\circ}$-Sn/Si(111) single atomic layer
Torkzadeh, Mohammadmehdi
Iannetti, Mattia
Lizée, Mathieu
Thakur, Amitayhush
Hervé, Maris
Debontridder, Francois
David, Pascal
Casula, Michele
Profeta, Gianni
Cren, Tristan
Calandra, Matteo
Tresca, Cesare
Brun, Christophe
Strongly Correlated Electrons
The one-third monolayer Sn layer on Si(111) has long been considered a benchmark system for exploring two-dimensional Mott physics, owing to its narrow bandwidth and sizable on-site Coulomb repulsion. Previous experiments suggested the emergence of a low-temperature Mott insulating phase with an energy gap of only a few tens of meV, while theory predicted a possible antiferromagnetic ordering that remained experimentally elusive. Here, by combining low-temperature scanning tunneling microscopy/spectroscopy with first-principles calculations, we reveal that the $\sqrt{3}\times\sqrt{3}$~R30$^{\circ}$-Sn/Si(111) surface undergoes a transition below 30K into a robust insulating state characterized by a remarkably large gap of about 440 $\pm$ 120 meV at 4K, five to ten times larger than previously reported. Quasiparticle interference imaging uncovers a well-defined $2\sqrt{3}\times\sqrt{3}$~R30$^{\circ}$-Sn/Si(111) superstructure, providing direct evidence for a two-dimensional stripe-like antiferromagnetic order. Ab initio calculations reveal that the silicon substrate stabilizes this phase through strong nonlocal tin-tin interactions, highlighting the decisive role of substrate-driven correlations in the $\sqrt{3}\times\sqrt{3}$~R30$^{\circ}$-Sn/Si(111) system.
title Antiferromagnetic stripe phase and large-gap insulating ground state of the correlated $\sqrt{3}\times\sqrt{3}$~R30$^{\circ}$-Sn/Si(111) single atomic layer
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2603.26304