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| Autori principali: | , , , , , , , , , , |
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| Natura: | Preprint |
| Pubblicazione: |
2026
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| Soggetti: | |
| Accesso online: | https://arxiv.org/abs/2603.26473 |
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| _version_ | 1866911548313698304 |
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| author | Torres-Boy, América Y. Ghosh, Anoushka Osenton, Myles B. T. Behera, Akash C. Gewinner, Sandy De Pas, Marco Junkes, Heinz Schöllkopf, Wieland Paarmann, Alexander von Helden, Gert Meijer, Gerard |
| author_facet | Torres-Boy, América Y. Ghosh, Anoushka Osenton, Myles B. T. Behera, Akash C. Gewinner, Sandy De Pas, Marco Junkes, Heinz Schöllkopf, Wieland Paarmann, Alexander von Helden, Gert Meijer, Gerard |
| contents | We report on the control and characterization of the isomer population of ions inside superfluid helium nanodroplets, using two-color operation of a dual-oscillator infrared free-electron laser. The timing of both lasers is highly synchronized, and their frequencies (or "colors") can be tuned independently over a wide range. Interaction of the singly deuterated proton-bound dimer of dihydrogen phosphate and formate inside helium nanodroplets with both colors enables the control over its isomer population and the recording of - one-color hidden - infrared spectra of individual isomers. |
| format | Preprint |
| id |
arxiv_https___arxiv_org_abs_2603_26473 |
| institution | arXiv |
| publishDate | 2026 |
| record_format | arxiv |
| spellingShingle | Controlling isomer population using a dual-oscillator infrared free-electron laser Torres-Boy, América Y. Ghosh, Anoushka Osenton, Myles B. T. Behera, Akash C. Gewinner, Sandy De Pas, Marco Junkes, Heinz Schöllkopf, Wieland Paarmann, Alexander von Helden, Gert Meijer, Gerard Chemical Physics We report on the control and characterization of the isomer population of ions inside superfluid helium nanodroplets, using two-color operation of a dual-oscillator infrared free-electron laser. The timing of both lasers is highly synchronized, and their frequencies (or "colors") can be tuned independently over a wide range. Interaction of the singly deuterated proton-bound dimer of dihydrogen phosphate and formate inside helium nanodroplets with both colors enables the control over its isomer population and the recording of - one-color hidden - infrared spectra of individual isomers. |
| title | Controlling isomer population using a dual-oscillator infrared free-electron laser |
| topic | Chemical Physics |
| url | https://arxiv.org/abs/2603.26473 |