Quantum transport reveals spin glass correlations in a 2D network of TbPc$_{2}$ single-molecule magnets grafted on graphene

Fuente: arXiv
Saved in:
Bibliographic Details
Main Authors: Wu, Nianjheng, Lefeuvre, Jules, Mayne, Andrew, Campidelli, Stéphane, Lagoute, Jérôme, Chacon, Cyril, Guéron, Sophie, Deblock, Richard, Bouchiat, Hélène
Format: Preprint
Published: 2026
Subjects:
Online Access:
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1866918419595526144
author Wu, Nianjheng
Lefeuvre, Jules
Mayne, Andrew
Campidelli, Stéphane
Lagoute, Jérôme
Chacon, Cyril
Guéron, Sophie
Deblock, Richard
Bouchiat, Hélène
author_facet Wu, Nianjheng
Lefeuvre, Jules
Mayne, Andrew
Campidelli, Stéphane
Lagoute, Jérôme
Chacon, Cyril
Guéron, Sophie
Deblock, Richard
Bouchiat, Hélène
contents The low temperature magnetoresistance of graphene functionalized by an array of magnetic Terbium Phthalocyanines molecules is found to exhibit a magnetic field-dependent 1/f noise, along with universal conductance fluctuations (UCFs) typical of a mesoscopic phase-coherent sample. A thorough analysis of the magnetic field, temperature and chemical potential dependence of this 1/f noise and UCFs reveals that long range, 2D Ising spin-glass like, magnetic correlations are induced in graphene through exchange interactions between the magnetic molecules and charge carriers in graphene. These experiments show that graphene functionalized with organic molecules constitutes a versatile platform for the investigation of magnetic phase transitions in two dimensions.
format Preprint
id arxiv_https___arxiv_org_abs_2603_29456
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Quantum transport reveals spin glass correlations in a 2D network of TbPc$_{2}$ single-molecule magnets grafted on graphene
Wu, Nianjheng
Lefeuvre, Jules
Mayne, Andrew
Campidelli, Stéphane
Lagoute, Jérôme
Chacon, Cyril
Guéron, Sophie
Deblock, Richard
Bouchiat, Hélène
Mesoscale and Nanoscale Physics
Disordered Systems and Neural Networks
The low temperature magnetoresistance of graphene functionalized by an array of magnetic Terbium Phthalocyanines molecules is found to exhibit a magnetic field-dependent 1/f noise, along with universal conductance fluctuations (UCFs) typical of a mesoscopic phase-coherent sample. A thorough analysis of the magnetic field, temperature and chemical potential dependence of this 1/f noise and UCFs reveals that long range, 2D Ising spin-glass like, magnetic correlations are induced in graphene through exchange interactions between the magnetic molecules and charge carriers in graphene. These experiments show that graphene functionalized with organic molecules constitutes a versatile platform for the investigation of magnetic phase transitions in two dimensions.
title Quantum transport reveals spin glass correlations in a 2D network of TbPc$_{2}$ single-molecule magnets grafted on graphene
topic Mesoscale and Nanoscale Physics
Disordered Systems and Neural Networks
url https://arxiv.org/abs/2603.29456