Detecting pairing symmetry of bilayer nickelates using electronic Raman scattering

Fuente: arXiv
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Hauptverfasser: Zhan, Jun, Bejas, Matías, Schnyder, Andreas P., Greco, Andrés, Wu, Xianxin, Hu, Jiangping
Format: Preprint
Veröffentlicht: 2026
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author Zhan, Jun
Bejas, Matías
Schnyder, Andreas P.
Greco, Andrés
Wu, Xianxin
Hu, Jiangping
author_facet Zhan, Jun
Bejas, Matías
Schnyder, Andreas P.
Greco, Andrés
Wu, Xianxin
Hu, Jiangping
contents The recent discovery of high-temperature superconductivity in both bulk and thin-film bilayer nickelates La$_3$Ni$_2$O$_7$ has garnered significant attention. However, the corresponding pairing symmetry remains debated in both experiments and theoretical studies due to conflicting experimental evidence from bulk and thin-film materials. In this work, we examine the electronic Raman response across different channels for various pairing symmetries within a two-orbital bilayer model. By comparing Raman susceptibilities obtained from multiorbital and band-additive approaches, we demonstrate that Raman response can distinguish between different pairing symmetries and identify pocket-dependent gap amplitudes for both fully gapped and nodal superconducting states. Specifically, the nodal $d_{x^2-y^2}/d_{xy}$-wave pairing exhibits robust low-energy power-law behavior, distinct from a fully gapped pairing. Additionally, for the $s_{\pm}$-wave pairing, the detailed gap anisotropy on the $β$ pocket can be determined. Possible experimental implications are also discussed. Our results highlight the crucial role of multiorbital effects in shaping the Raman spectra and establish electronic Raman scattering as a powerful and symmetry-resolved probe for determining the superconducting gap in unconventional superconductors.
format Preprint
id arxiv_https___arxiv_org_abs_2604_01027
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Detecting pairing symmetry of bilayer nickelates using electronic Raman scattering
Zhan, Jun
Bejas, Matías
Schnyder, Andreas P.
Greco, Andrés
Wu, Xianxin
Hu, Jiangping
Superconductivity
The recent discovery of high-temperature superconductivity in both bulk and thin-film bilayer nickelates La$_3$Ni$_2$O$_7$ has garnered significant attention. However, the corresponding pairing symmetry remains debated in both experiments and theoretical studies due to conflicting experimental evidence from bulk and thin-film materials. In this work, we examine the electronic Raman response across different channels for various pairing symmetries within a two-orbital bilayer model. By comparing Raman susceptibilities obtained from multiorbital and band-additive approaches, we demonstrate that Raman response can distinguish between different pairing symmetries and identify pocket-dependent gap amplitudes for both fully gapped and nodal superconducting states. Specifically, the nodal $d_{x^2-y^2}/d_{xy}$-wave pairing exhibits robust low-energy power-law behavior, distinct from a fully gapped pairing. Additionally, for the $s_{\pm}$-wave pairing, the detailed gap anisotropy on the $β$ pocket can be determined. Possible experimental implications are also discussed. Our results highlight the crucial role of multiorbital effects in shaping the Raman spectra and establish electronic Raman scattering as a powerful and symmetry-resolved probe for determining the superconducting gap in unconventional superconductors.
title Detecting pairing symmetry of bilayer nickelates using electronic Raman scattering
topic Superconductivity
url https://arxiv.org/abs/2604.01027