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Main Authors: Yu, Zhongwei, Tutunov, Rasul, Maraval, Alexandre Max, Xie, Zikai, Tan, Zhenzhi, Wang, Jiankang, Cao, Bin, Li, Zijing, Xu, Liangliang, Yang, Qi, Jiang, Jun, Luo, Sanzhong, Guo, Zhenxiao, Zhang, Tongyi, Bou-Ammar, Haitham, Wang, Jun
Format: Preprint
Published: 2026
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Online Access:https://arxiv.org/abs/2604.01328
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author Yu, Zhongwei
Tutunov, Rasul
Maraval, Alexandre Max
Xie, Zikai
Tan, Zhenzhi
Wang, Jiankang
Cao, Bin
Li, Zijing
Xu, Liangliang
Yang, Qi
Jiang, Jun
Luo, Sanzhong
Guo, Zhenxiao
Zhang, Tongyi
Bou-Ammar, Haitham
Wang, Jun
author_facet Yu, Zhongwei
Tutunov, Rasul
Maraval, Alexandre Max
Xie, Zikai
Tan, Zhenzhi
Wang, Jiankang
Cao, Bin
Li, Zijing
Xu, Liangliang
Yang, Qi
Jiang, Jun
Luo, Sanzhong
Guo, Zhenxiao
Zhang, Tongyi
Bou-Ammar, Haitham
Wang, Jun
contents Traditional scientific discovery relies on an iterative hypothesise-experiment-refine cycle that has driven progress for centuries, but its intuitive, ad-hoc implementation often wastes resources, yields inefficient designs, and misses critical insights. This tutorial presents Bayesian Optimisation (BO), a principled probability-driven framework that formalises and automates this core scientific cycle. BO uses surrogate models (e.g., Gaussian processes) to model empirical observations as evolving hypotheses, and acquisition functions to guide experiment selection, balancing exploitation of known knowledge and exploration of uncharted domains to eliminate guesswork and manual trial-and-error. We first frame scientific discovery as an optimisation problem, then unpack BO's core components, end-to-end workflows, and real-world efficacy via case studies in catalysis, materials science, organic synthesis, and molecule discovery. We also cover critical technical extensions for scientific applications, including batched experimentation, heteroscedasticity, contextual optimisation, and human-in-the-loop integration. Tailored for a broad audience, this tutorial bridges AI advances in BO with practical natural science applications, offering tiered content to empower cross-disciplinary researchers to design more efficient experiments and accelerate principled scientific discovery.
format Preprint
id arxiv_https___arxiv_org_abs_2604_01328
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Efficient and Principled Scientific Discovery through Bayesian Optimization: A Tutorial
Yu, Zhongwei
Tutunov, Rasul
Maraval, Alexandre Max
Xie, Zikai
Tan, Zhenzhi
Wang, Jiankang
Cao, Bin
Li, Zijing
Xu, Liangliang
Yang, Qi
Jiang, Jun
Luo, Sanzhong
Guo, Zhenxiao
Zhang, Tongyi
Bou-Ammar, Haitham
Wang, Jun
Machine Learning
Traditional scientific discovery relies on an iterative hypothesise-experiment-refine cycle that has driven progress for centuries, but its intuitive, ad-hoc implementation often wastes resources, yields inefficient designs, and misses critical insights. This tutorial presents Bayesian Optimisation (BO), a principled probability-driven framework that formalises and automates this core scientific cycle. BO uses surrogate models (e.g., Gaussian processes) to model empirical observations as evolving hypotheses, and acquisition functions to guide experiment selection, balancing exploitation of known knowledge and exploration of uncharted domains to eliminate guesswork and manual trial-and-error. We first frame scientific discovery as an optimisation problem, then unpack BO's core components, end-to-end workflows, and real-world efficacy via case studies in catalysis, materials science, organic synthesis, and molecule discovery. We also cover critical technical extensions for scientific applications, including batched experimentation, heteroscedasticity, contextual optimisation, and human-in-the-loop integration. Tailored for a broad audience, this tutorial bridges AI advances in BO with practical natural science applications, offering tiered content to empower cross-disciplinary researchers to design more efficient experiments and accelerate principled scientific discovery.
title Efficient and Principled Scientific Discovery through Bayesian Optimization: A Tutorial
topic Machine Learning
url https://arxiv.org/abs/2604.01328