Valence Bond Glass and Glassy Spin Liquid in Disordered Frustrated Magnets

Fuente: arXiv
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Autori principali: Dash, Soumyaranjan, Narang, Vansh, Kumar, Sanjeev
Natura: Preprint
Pubblicazione: 2026
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author Dash, Soumyaranjan
Narang, Vansh
Kumar, Sanjeev
author_facet Dash, Soumyaranjan
Narang, Vansh
Kumar, Sanjeev
contents The absence of conventional magnetic order together with anomalous low-temperature magnetic heat capacity is often interpreted as evidence for quantum spin liquid ground states in frustrated magnets. Using a recently developed semiclassical Monte Carlo approach, we show that similar thermodynamic signatures arise in the highly frustrated regime of the disordered spin-1/2 J1-J2 Heisenberg model on the square lattice. By analyzing the freezing parameters, the distribution of spin-spin correlations, and the specific heat, we identify the ground state as a valence-bond glass that melts into a glassy spin liquid at finite temperatures. We show that the low-temperature specific-heat anomaly originates from collective singlet excitations, and consequently it is insensitive to external magnetic fields. This leads to a robust experimental signature of the valence bond glass phase and a completely new interpretation of the thermodynamic data on disordered spin-liquid candidate materials.
format Preprint
id arxiv_https___arxiv_org_abs_2604_05501
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Valence Bond Glass and Glassy Spin Liquid in Disordered Frustrated Magnets
Dash, Soumyaranjan
Narang, Vansh
Kumar, Sanjeev
Strongly Correlated Electrons
The absence of conventional magnetic order together with anomalous low-temperature magnetic heat capacity is often interpreted as evidence for quantum spin liquid ground states in frustrated magnets. Using a recently developed semiclassical Monte Carlo approach, we show that similar thermodynamic signatures arise in the highly frustrated regime of the disordered spin-1/2 J1-J2 Heisenberg model on the square lattice. By analyzing the freezing parameters, the distribution of spin-spin correlations, and the specific heat, we identify the ground state as a valence-bond glass that melts into a glassy spin liquid at finite temperatures. We show that the low-temperature specific-heat anomaly originates from collective singlet excitations, and consequently it is insensitive to external magnetic fields. This leads to a robust experimental signature of the valence bond glass phase and a completely new interpretation of the thermodynamic data on disordered spin-liquid candidate materials.
title Valence Bond Glass and Glassy Spin Liquid in Disordered Frustrated Magnets
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2604.05501