Ultrafast nonlinear Hall effect in black phosphorus

Fuente: arXiv
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Main Authors: Dendzik, Maciej, Marini, Andrea, Beaulieu, Samuel, Dong, Shuo, Pincelli, Tommaso, Maklar, Julian, Xian, R. Patrick, Perfetto, Enrico, Wolf, Martin, Stefanucci, Gianluca, Ernstorfer, Ralph, Rettig, Laurenz
Format: Preprint
Published: 2026
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author Dendzik, Maciej
Marini, Andrea
Beaulieu, Samuel
Dong, Shuo
Pincelli, Tommaso
Maklar, Julian
Xian, R. Patrick
Perfetto, Enrico
Wolf, Martin
Stefanucci, Gianluca
Ernstorfer, Ralph
Rettig, Laurenz
author_facet Dendzik, Maciej
Marini, Andrea
Beaulieu, Samuel
Dong, Shuo
Pincelli, Tommaso
Maklar, Julian
Xian, R. Patrick
Perfetto, Enrico
Wolf, Martin
Stefanucci, Gianluca
Ernstorfer, Ralph
Rettig, Laurenz
contents The nonlinear Hall effect (NHE) is a recently discovered member of the Hall effect family in which the Hall voltage shows a nonlinear behavior when a transverse electric field is applied. While the NHE does not require broken time-reversal symmetry, such as that induced by a magnetic field, it requires broken inversion symmetry, which limits the range of suitable systems and potential applications. Here, we demonstrate an ultrafast NHE in centrosymmetric black phosphorus through dynamical symmetry breaking using femtosecond light pulses. We provide a detailed microscopic picture of excited carrier dynamics and induced fields using momentum-resolved photoemission spectroscopy combined with \textit{ab-initio} calculations. The ultrafast NHE is observed exclusively for the light polarization aligned with the armchair high-symmetry direction and persists over 300 fs, which opens new possibilities for selective and ultrafast light-to-current conversions.
format Preprint
id arxiv_https___arxiv_org_abs_2604_06083
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Ultrafast nonlinear Hall effect in black phosphorus
Dendzik, Maciej
Marini, Andrea
Beaulieu, Samuel
Dong, Shuo
Pincelli, Tommaso
Maklar, Julian
Xian, R. Patrick
Perfetto, Enrico
Wolf, Martin
Stefanucci, Gianluca
Ernstorfer, Ralph
Rettig, Laurenz
Materials Science
Mesoscale and Nanoscale Physics
Strongly Correlated Electrons
The nonlinear Hall effect (NHE) is a recently discovered member of the Hall effect family in which the Hall voltage shows a nonlinear behavior when a transverse electric field is applied. While the NHE does not require broken time-reversal symmetry, such as that induced by a magnetic field, it requires broken inversion symmetry, which limits the range of suitable systems and potential applications. Here, we demonstrate an ultrafast NHE in centrosymmetric black phosphorus through dynamical symmetry breaking using femtosecond light pulses. We provide a detailed microscopic picture of excited carrier dynamics and induced fields using momentum-resolved photoemission spectroscopy combined with \textit{ab-initio} calculations. The ultrafast NHE is observed exclusively for the light polarization aligned with the armchair high-symmetry direction and persists over 300 fs, which opens new possibilities for selective and ultrafast light-to-current conversions.
title Ultrafast nonlinear Hall effect in black phosphorus
topic Materials Science
Mesoscale and Nanoscale Physics
Strongly Correlated Electrons
url https://arxiv.org/abs/2604.06083