Ten-Second Electron-Spin Coherence in Isotopically Engineered Diamond

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Hauptverfasser: Yamamoto, Takashi, van Ommen, H. Benjamin, Schymik, Kai-Niklas, de Zoeten, Beer, Onoda, Shinobu, Saiki, Seiichi, Ohshima, Takeshi, Arjmandi-Tash, Hadi, Vollmer, René, Taminiau, Tim H.
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Veröffentlicht: 2026
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author Yamamoto, Takashi
van Ommen, H. Benjamin
Schymik, Kai-Niklas
de Zoeten, Beer
Onoda, Shinobu
Saiki, Seiichi
Ohshima, Takeshi
Arjmandi-Tash, Hadi
Vollmer, René
Taminiau, Tim H.
author_facet Yamamoto, Takashi
van Ommen, H. Benjamin
Schymik, Kai-Niklas
de Zoeten, Beer
Onoda, Shinobu
Saiki, Seiichi
Ohshima, Takeshi
Arjmandi-Tash, Hadi
Vollmer, René
Taminiau, Tim H.
contents Solid-state spin defects are a promising platform for quantum networks. A key requirement is to combine long ground-state spin-coherence times with a coherent optical transition for spin-photon entanglement. Here, we investigate the spin and optical coherence of single nitrogen-vacancy (NV) centres in (111)-grown isotopically engineered diamond. Our diamond-growth process yields a precisely controlled $^{13}\mathrm{C}$ concentration and low-ppb nitrogen concentrations. Combined with the mitigation of 50 Hz noise using a real-time feedforward scheme and tailored decoupling sequences, this enables record defect-electron-spin coherence times of $T_2 = 6.8(1)$ ms for a Hahn echo and of $T_2^{DD} = 11.2(8)$ s under dynamical decoupling. In addition, we observe coherent optical transitions with a near-lifetime-limited homogeneous linewidth of 16.9(4) MHz and characterize the spectral diffusion dynamics. These results provide new avenues to investigate the incorporation of impurities in diamond and new opportunities for improved spin-qubit control for quantum networks and other quantum technologies.
format Preprint
id arxiv_https___arxiv_org_abs_2604_07439
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Ten-Second Electron-Spin Coherence in Isotopically Engineered Diamond
Yamamoto, Takashi
van Ommen, H. Benjamin
Schymik, Kai-Niklas
de Zoeten, Beer
Onoda, Shinobu
Saiki, Seiichi
Ohshima, Takeshi
Arjmandi-Tash, Hadi
Vollmer, René
Taminiau, Tim H.
Quantum Physics
Solid-state spin defects are a promising platform for quantum networks. A key requirement is to combine long ground-state spin-coherence times with a coherent optical transition for spin-photon entanglement. Here, we investigate the spin and optical coherence of single nitrogen-vacancy (NV) centres in (111)-grown isotopically engineered diamond. Our diamond-growth process yields a precisely controlled $^{13}\mathrm{C}$ concentration and low-ppb nitrogen concentrations. Combined with the mitigation of 50 Hz noise using a real-time feedforward scheme and tailored decoupling sequences, this enables record defect-electron-spin coherence times of $T_2 = 6.8(1)$ ms for a Hahn echo and of $T_2^{DD} = 11.2(8)$ s under dynamical decoupling. In addition, we observe coherent optical transitions with a near-lifetime-limited homogeneous linewidth of 16.9(4) MHz and characterize the spectral diffusion dynamics. These results provide new avenues to investigate the incorporation of impurities in diamond and new opportunities for improved spin-qubit control for quantum networks and other quantum technologies.
title Ten-Second Electron-Spin Coherence in Isotopically Engineered Diamond
topic Quantum Physics
url https://arxiv.org/abs/2604.07439