Giant photostriction in lead-free ferroelectric stemming from photo-excited thermalized carriers
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arXiv
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| Auteurs principaux: | , , , , , , , , , , , , , , , , |
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| Format: | Preprint |
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2026
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| _version_ | 1866917395595001856 |
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| author | Vitali-Derrien, Gaëlle Condurache, Oana Ducournau, Antoine Gemeiner, Pascale Vallet, Maxime Guiblin, Nicolas Antoni, Thomas Matzen, Sylvia Ruello, Pascal Chvostova, Dagmar Ostapchuk, Tetyana Hlinka, Jirka Hurand, Simon Khiari, Mouna Bouyanfif, Houssny Paillard, Charles Janolin, Pierre-Eymeric |
| author_facet | Vitali-Derrien, Gaëlle Condurache, Oana Ducournau, Antoine Gemeiner, Pascale Vallet, Maxime Guiblin, Nicolas Antoni, Thomas Matzen, Sylvia Ruello, Pascal Chvostova, Dagmar Ostapchuk, Tetyana Hlinka, Jirka Hurand, Simon Khiari, Mouna Bouyanfif, Houssny Paillard, Charles Janolin, Pierre-Eymeric |
| contents | Ferroelectrics are polar materials whose polarization can be switched by applying electric fields; they offer unique opportunities to develop performant photostrictive materials, i.e., materials that can deform under visible light illumination. Naturally devoid of inversion symmetry, they exhibit original photogalvanic effects such as the Bulk Photovoltaic Effect, which relies on ``hot'' photoexcited carriers. It has long been thought that the electric field generated by this effect may couple to the natural piezoelectric abilities of ferroelectrics to provide large photoinduced deformations. However, due to competing effects, such as thermal dilatation, deformation potential, polarization, or depolarizing-field screening by \textit{thermalized} carriers, it remains unclear which microscopic phenomena govern the photoinduced deformations in classical ferroelectric materials. Here, we demonstrate the largest photoinduced deformation measured in a ferroelectric thin film. Reaching 1 %, this giant photostriction likely originates from the contribution of thermalized photoinduced carriers. |
| format | Preprint |
| id |
arxiv_https___arxiv_org_abs_2604_08218 |
| institution | arXiv |
| publishDate | 2026 |
| record_format | arxiv |
| spellingShingle | Giant photostriction in lead-free ferroelectric stemming from photo-excited thermalized carriers Vitali-Derrien, Gaëlle Condurache, Oana Ducournau, Antoine Gemeiner, Pascale Vallet, Maxime Guiblin, Nicolas Antoni, Thomas Matzen, Sylvia Ruello, Pascal Chvostova, Dagmar Ostapchuk, Tetyana Hlinka, Jirka Hurand, Simon Khiari, Mouna Bouyanfif, Houssny Paillard, Charles Janolin, Pierre-Eymeric Materials Science Ferroelectrics are polar materials whose polarization can be switched by applying electric fields; they offer unique opportunities to develop performant photostrictive materials, i.e., materials that can deform under visible light illumination. Naturally devoid of inversion symmetry, they exhibit original photogalvanic effects such as the Bulk Photovoltaic Effect, which relies on ``hot'' photoexcited carriers. It has long been thought that the electric field generated by this effect may couple to the natural piezoelectric abilities of ferroelectrics to provide large photoinduced deformations. However, due to competing effects, such as thermal dilatation, deformation potential, polarization, or depolarizing-field screening by \textit{thermalized} carriers, it remains unclear which microscopic phenomena govern the photoinduced deformations in classical ferroelectric materials. Here, we demonstrate the largest photoinduced deformation measured in a ferroelectric thin film. Reaching 1 %, this giant photostriction likely originates from the contribution of thermalized photoinduced carriers. |
| title | Giant photostriction in lead-free ferroelectric stemming from photo-excited thermalized carriers |
| topic | Materials Science |
| url | https://arxiv.org/abs/2604.08218 |