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Auteurs principaux: Ning, Ruo-Yu, Wang, Yong-Kun, Qian, Shifeng, Li, Si, Yang, Wen-Li
Format: Preprint
Publié: 2026
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Accès en ligne:https://arxiv.org/abs/2604.08907
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author Ning, Ruo-Yu
Wang, Yong-Kun
Qian, Shifeng
Li, Si
Yang, Wen-Li
author_facet Ning, Ruo-Yu
Wang, Yong-Kun
Qian, Shifeng
Li, Si
Yang, Wen-Li
contents Based on first-principles calculations combined with theoretical analysis, we identify a family of monolayer chromium-based group-IV chalcogenides as a new class of two-dimensional (2D) magnetic higher-order topological insulators (HOTIs). Specifically, the CrC$X_3$ ($X=$ S, Se, Te) and CrSiS$_3$ monolayers are found to host conventional antiferromagnetic ground states with $\mathcal{PT}$ symmetry, whereas the Janus compounds Cr$_2$C$_2$S$_3$Se$_3$ and Cr$_2$Si$_2$S$_3$Se$_3$ exhibit altermagnetic ground states. We demonstrate that all these monolayer magnetic materials realize 2D HOTI phases, in which the nontrivial topology is protected by lattice $C_3$ rotational symmetry and manifests as zero-dimensional corner states carrying quantized fractional charges. Moreover, upon inclusion of spin-orbit coupling, these systems remain in the HOTI phase and continue to host robust corner-localized states, confirming the stability of their higher-order topological nature. Our results reveal an intrinsic connection between higher-order topology and magnetic order in 2D antiferromagnetic and altermagnetic systems, identifying chromium-based group-IV chalcogenide monolayers as promising platforms for exploring higher-order topological phases and their potential relevance for future topological and spintronic applications.
format Preprint
id arxiv_https___arxiv_org_abs_2604_08907
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Higher-order topological insulators in two-dimensional antiferromagnetic and altermagnetic chromium-based group-IV chalcogenides
Ning, Ruo-Yu
Wang, Yong-Kun
Qian, Shifeng
Li, Si
Yang, Wen-Li
Materials Science
Based on first-principles calculations combined with theoretical analysis, we identify a family of monolayer chromium-based group-IV chalcogenides as a new class of two-dimensional (2D) magnetic higher-order topological insulators (HOTIs). Specifically, the CrC$X_3$ ($X=$ S, Se, Te) and CrSiS$_3$ monolayers are found to host conventional antiferromagnetic ground states with $\mathcal{PT}$ symmetry, whereas the Janus compounds Cr$_2$C$_2$S$_3$Se$_3$ and Cr$_2$Si$_2$S$_3$Se$_3$ exhibit altermagnetic ground states. We demonstrate that all these monolayer magnetic materials realize 2D HOTI phases, in which the nontrivial topology is protected by lattice $C_3$ rotational symmetry and manifests as zero-dimensional corner states carrying quantized fractional charges. Moreover, upon inclusion of spin-orbit coupling, these systems remain in the HOTI phase and continue to host robust corner-localized states, confirming the stability of their higher-order topological nature. Our results reveal an intrinsic connection between higher-order topology and magnetic order in 2D antiferromagnetic and altermagnetic systems, identifying chromium-based group-IV chalcogenide monolayers as promising platforms for exploring higher-order topological phases and their potential relevance for future topological and spintronic applications.
title Higher-order topological insulators in two-dimensional antiferromagnetic and altermagnetic chromium-based group-IV chalcogenides
topic Materials Science
url https://arxiv.org/abs/2604.08907