NaCl-Assisted Growth of Ferroelectric SnSe Nanosheets with Spin Glass-like Behavior

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Hauptverfasser: Xu, Huiwen, Wu, Hanxiang, Li, Chang, Pang, Fei
Format: Preprint
Veröffentlicht: 2026
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author Xu, Huiwen
Wu, Hanxiang
Li, Chang
Pang, Fei
author_facet Xu, Huiwen
Wu, Hanxiang
Li, Chang
Pang, Fei
contents Two-dimensional (2D) SnSe is an emerging 2D material exhibiting intriguing properties such as ferroelectricity and nonlinear optical response. Here, high-quality single-crystalline SnSe nanosheets were synthesized via NaCl-assisted chemical vapor deposition (CVD) method. The addition of NaCl was found to significantly increase the surface coverage of the nanosheets with less influence on their lateral size. The crystalline structure and composition of as-grown nanosheets were charactered by XRD, Raman spectroscopy, and XPS. Ferroelectric domains in SnSe nanosheets are directly visualized by piezoresponse force microscopy (PFM). The magnetic hysteresis loops of SnSe nanosheets are achieved at 2 K, which indicated their weak ferromagnetism. A spin glass-like behavior was observed below 115K, which is attributed to the presence of SnSe2 impurity. This work further establishes a controllable synthesis route for SnSe nanosheets, thereby paving the way for subsequent investigation of their ferroelectric properties.
format Preprint
id arxiv_https___arxiv_org_abs_2604_10067
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle NaCl-Assisted Growth of Ferroelectric SnSe Nanosheets with Spin Glass-like Behavior
Xu, Huiwen
Wu, Hanxiang
Li, Chang
Pang, Fei
Materials Science
Mesoscale and Nanoscale Physics
Two-dimensional (2D) SnSe is an emerging 2D material exhibiting intriguing properties such as ferroelectricity and nonlinear optical response. Here, high-quality single-crystalline SnSe nanosheets were synthesized via NaCl-assisted chemical vapor deposition (CVD) method. The addition of NaCl was found to significantly increase the surface coverage of the nanosheets with less influence on their lateral size. The crystalline structure and composition of as-grown nanosheets were charactered by XRD, Raman spectroscopy, and XPS. Ferroelectric domains in SnSe nanosheets are directly visualized by piezoresponse force microscopy (PFM). The magnetic hysteresis loops of SnSe nanosheets are achieved at 2 K, which indicated their weak ferromagnetism. A spin glass-like behavior was observed below 115K, which is attributed to the presence of SnSe2 impurity. This work further establishes a controllable synthesis route for SnSe nanosheets, thereby paving the way for subsequent investigation of their ferroelectric properties.
title NaCl-Assisted Growth of Ferroelectric SnSe Nanosheets with Spin Glass-like Behavior
topic Materials Science
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2604.10067