2D quantum-path interference in high-harmonic generation driven by highly-bichromatic fields

Fuente: arXiv
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Main Authors: Zou, Xiaozhou, Jurkovičová, Lucie, Weber, Anne, Zhao, Cong, Albrecht, Martin, Finke, Ondřej, Vendl, Alexandr, Grenfell, Annika, Szuba, Wojciech, Nejdl, Jaroslav, Constant, Eric, Khokhlova, Margarita, Pisanty, Emilio, Hort, Ondřej, Zaïr, Amelle
Format: Preprint
Published: 2026
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author Zou, Xiaozhou
Jurkovičová, Lucie
Weber, Anne
Zhao, Cong
Albrecht, Martin
Finke, Ondřej
Vendl, Alexandr
Grenfell, Annika
Szuba, Wojciech
Nejdl, Jaroslav
Constant, Eric
Khokhlova, Margarita
Pisanty, Emilio
Hort, Ondřej
Zaïr, Amelle
author_facet Zou, Xiaozhou
Jurkovičová, Lucie
Weber, Anne
Zhao, Cong
Albrecht, Martin
Finke, Ondřej
Vendl, Alexandr
Grenfell, Annika
Szuba, Wojciech
Nejdl, Jaroslav
Constant, Eric
Khokhlova, Margarita
Pisanty, Emilio
Hort, Ondřej
Zaïr, Amelle
contents We experimentally observe a new type of quantum-path interference, in two-dimensions (2D-QPI), in high-harmonic generation (HHG) driven by an orthogonally-polarised highly-bichromatic field. This regime is marked by comparable intensities of the two orthogonal colours. In this highly-bichromatic regime, we demonstrate that 2D-QPI is encoded in the measured harmonic intensity modulations with respect to the relative phase of the two-colour field. The modulations of the odd-order harmonics show a monomodal behaviour, whereas the even harmonics are modulated in a bimodal structure. Our calculations using the strong-field approximation and saddle-point method disentangle contributions from multiple quantum orbits in this HHG regime, revealing that the dipole response for both odd and even harmonics inherits the dynamic symmetry of the orthogonally-polarised driving field. This new type of 2D-QPI offers a novel route to HHG spectroscopy of attosecond electron dynamics by lifting up the dimensionality of the quantum paths involved in the interference.
format Preprint
id arxiv_https___arxiv_org_abs_2604_12838
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle 2D quantum-path interference in high-harmonic generation driven by highly-bichromatic fields
Zou, Xiaozhou
Jurkovičová, Lucie
Weber, Anne
Zhao, Cong
Albrecht, Martin
Finke, Ondřej
Vendl, Alexandr
Grenfell, Annika
Szuba, Wojciech
Nejdl, Jaroslav
Constant, Eric
Khokhlova, Margarita
Pisanty, Emilio
Hort, Ondřej
Zaïr, Amelle
Quantum Physics
Optics
We experimentally observe a new type of quantum-path interference, in two-dimensions (2D-QPI), in high-harmonic generation (HHG) driven by an orthogonally-polarised highly-bichromatic field. This regime is marked by comparable intensities of the two orthogonal colours. In this highly-bichromatic regime, we demonstrate that 2D-QPI is encoded in the measured harmonic intensity modulations with respect to the relative phase of the two-colour field. The modulations of the odd-order harmonics show a monomodal behaviour, whereas the even harmonics are modulated in a bimodal structure. Our calculations using the strong-field approximation and saddle-point method disentangle contributions from multiple quantum orbits in this HHG regime, revealing that the dipole response for both odd and even harmonics inherits the dynamic symmetry of the orthogonally-polarised driving field. This new type of 2D-QPI offers a novel route to HHG spectroscopy of attosecond electron dynamics by lifting up the dimensionality of the quantum paths involved in the interference.
title 2D quantum-path interference in high-harmonic generation driven by highly-bichromatic fields
topic Quantum Physics
Optics
url https://arxiv.org/abs/2604.12838