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Main Authors: Hollendonner, Maximilian, Hrunski, Fedor Dzmitryevich, Scheller, Daniel, Ullerich, Kim, Parthasarathy, Shravan Kumar, Knolle, Wolfgang, Schober, Maximilian, Neubauer, Mirjam, Dasari, Durga Bhaktavatsala Rao, Bockstedte, Michel, Nagy, Roland
Format: Preprint
Published: 2026
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Online Access:https://arxiv.org/abs/2604.16194
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author Hollendonner, Maximilian
Hrunski, Fedor Dzmitryevich
Scheller, Daniel
Ullerich, Kim
Parthasarathy, Shravan Kumar
Knolle, Wolfgang
Schober, Maximilian
Neubauer, Mirjam
Dasari, Durga Bhaktavatsala Rao
Bockstedte, Michel
Nagy, Roland
author_facet Hollendonner, Maximilian
Hrunski, Fedor Dzmitryevich
Scheller, Daniel
Ullerich, Kim
Parthasarathy, Shravan Kumar
Knolle, Wolfgang
Schober, Maximilian
Neubauer, Mirjam
Dasari, Durga Bhaktavatsala Rao
Bockstedte, Michel
Nagy, Roland
contents Silicon vacancy (VSi) centers in 4H silicon carbide have emerged as a highly promising platform for semiconductor-based quantum technologies, combining excellent spin and optical properties with an industrial-grade, CMOS-compatible material. As these defects are increasingly integrated into practical quantum devices, they inevitably encounter lattice strain. However, while the impact of strain is well documented for other solid-state defects like NV centers in diamond, its specific influence on key VSi spin dynamics such as initialization fidelity and state lifetimes remain largely unexplored. In this work, we address this critical gap by designing fully optical pulse sequences and incorporating the effective spin-3/2 strain Hamiltonian into our analysis. This combined approach allows us to isolate both axial and transverse strain contributions and systematically characterize their effect on the metastable state transition rates. Specifically, we reveal that strain significantly reduces the transition rates from the energetically lowest metastable state to the ground state quartet, leading to decreased photon emission. Supported by first-principles calculations, our findings provide a deeper understanding of VSi spin-strain dynamics, yielding crucial insights for the robust deployment of these centers in realistic, strain-prone environments.
format Preprint
id arxiv_https___arxiv_org_abs_2604_16194
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Strain-induced modification of spin-optical dynamics in silicon vacancy centers for integrated quantum technologies
Hollendonner, Maximilian
Hrunski, Fedor Dzmitryevich
Scheller, Daniel
Ullerich, Kim
Parthasarathy, Shravan Kumar
Knolle, Wolfgang
Schober, Maximilian
Neubauer, Mirjam
Dasari, Durga Bhaktavatsala Rao
Bockstedte, Michel
Nagy, Roland
Quantum Physics
Silicon vacancy (VSi) centers in 4H silicon carbide have emerged as a highly promising platform for semiconductor-based quantum technologies, combining excellent spin and optical properties with an industrial-grade, CMOS-compatible material. As these defects are increasingly integrated into practical quantum devices, they inevitably encounter lattice strain. However, while the impact of strain is well documented for other solid-state defects like NV centers in diamond, its specific influence on key VSi spin dynamics such as initialization fidelity and state lifetimes remain largely unexplored. In this work, we address this critical gap by designing fully optical pulse sequences and incorporating the effective spin-3/2 strain Hamiltonian into our analysis. This combined approach allows us to isolate both axial and transverse strain contributions and systematically characterize their effect on the metastable state transition rates. Specifically, we reveal that strain significantly reduces the transition rates from the energetically lowest metastable state to the ground state quartet, leading to decreased photon emission. Supported by first-principles calculations, our findings provide a deeper understanding of VSi spin-strain dynamics, yielding crucial insights for the robust deployment of these centers in realistic, strain-prone environments.
title Strain-induced modification of spin-optical dynamics in silicon vacancy centers for integrated quantum technologies
topic Quantum Physics
url https://arxiv.org/abs/2604.16194