Static and Dynamic Electronic Properties and the Possible Magnetic Structure of the $4f^3$-$Γ_6$ System NdCo2Zn$_{18}$Ga$_2$ Investigated Using $^{59}$Co Nuclear Quadrupole Resonance

Fuente: arXiv
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Main Authors: Kubo, Tetsuro, Sasaki, Atsushi, Murooka, Keita, Kotegawa, Hisashi, Yamamoto, Rikako, Onimaru, Takahiro, Tou, Hideki
Format: Preprint
Published: 2026
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_version_ 1866917420535382016
author Kubo, Tetsuro
Sasaki, Atsushi
Murooka, Keita
Kotegawa, Hisashi
Yamamoto, Rikako
Onimaru, Takahiro
Tou, Hideki
author_facet Kubo, Tetsuro
Sasaki, Atsushi
Murooka, Keita
Kotegawa, Hisashi
Yamamoto, Rikako
Onimaru, Takahiro
Tou, Hideki
contents We report $^{59}$Co nuclear quadrupole resonance (NQR) measurements on the Nd-based compound NdCo$_2$Zn$_{18}$Ga$_2$, which undergoes an antiferromagnetic transition at $T_{\rm N} = 1.5$ K. Although the NQR spectra show no detectable change across $T_{\rm N}$, the nuclear spin-lattice relaxation rate, $1/T_1$, exhibits a clear anomaly at $T_{\rm N}$. An analysis based on the alignment of the Nd moments demonstrates that the internal magnetic fields generated by these moments cancel each other at the Co sites. If the nearest-neighbor Nd moments align antiferromagnetically, this finding suggests that Ga substitution removes magnetic frustration, thereby increasing $T_{\rm N}$.
format Preprint
id arxiv_https___arxiv_org_abs_2604_17416
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Static and Dynamic Electronic Properties and the Possible Magnetic Structure of the $4f^3$-$Γ_6$ System NdCo2Zn$_{18}$Ga$_2$ Investigated Using $^{59}$Co Nuclear Quadrupole Resonance
Kubo, Tetsuro
Sasaki, Atsushi
Murooka, Keita
Kotegawa, Hisashi
Yamamoto, Rikako
Onimaru, Takahiro
Tou, Hideki
Strongly Correlated Electrons
We report $^{59}$Co nuclear quadrupole resonance (NQR) measurements on the Nd-based compound NdCo$_2$Zn$_{18}$Ga$_2$, which undergoes an antiferromagnetic transition at $T_{\rm N} = 1.5$ K. Although the NQR spectra show no detectable change across $T_{\rm N}$, the nuclear spin-lattice relaxation rate, $1/T_1$, exhibits a clear anomaly at $T_{\rm N}$. An analysis based on the alignment of the Nd moments demonstrates that the internal magnetic fields generated by these moments cancel each other at the Co sites. If the nearest-neighbor Nd moments align antiferromagnetically, this finding suggests that Ga substitution removes magnetic frustration, thereby increasing $T_{\rm N}$.
title Static and Dynamic Electronic Properties and the Possible Magnetic Structure of the $4f^3$-$Γ_6$ System NdCo2Zn$_{18}$Ga$_2$ Investigated Using $^{59}$Co Nuclear Quadrupole Resonance
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2604.17416