Proximity Magnetism in Mn(Bi,Sb)2Te4-(Bi,Sb)2Te3/MnTe Natural Heterostructures

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Hauptverfasser: Vail, Owen A., Wang, Shu-Wei, Hou, Yasen, Hettiarachchi, Dinura, Milette, Jean-Felix, Eldred, Tim B., Gao, Wenpei, Sarney, Wendy, Ambaye, Haile, Keum, Jong, Lauter, Valeria, de Coster, George J., Gilbert, Matthew J., Heiman, Don, Moodera, Jagadeesh S., Chi, Hang
Format: Preprint
Veröffentlicht: 2026
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author Vail, Owen A.
Wang, Shu-Wei
Hou, Yasen
Hettiarachchi, Dinura
Milette, Jean-Felix
Eldred, Tim B.
Gao, Wenpei
Sarney, Wendy
Ambaye, Haile
Keum, Jong
Lauter, Valeria
de Coster, George J.
Gilbert, Matthew J.
Heiman, Don
Moodera, Jagadeesh S.
Chi, Hang
author_facet Vail, Owen A.
Wang, Shu-Wei
Hou, Yasen
Hettiarachchi, Dinura
Milette, Jean-Felix
Eldred, Tim B.
Gao, Wenpei
Sarney, Wendy
Ambaye, Haile
Keum, Jong
Lauter, Valeria
de Coster, George J.
Gilbert, Matthew J.
Heiman, Don
Moodera, Jagadeesh S.
Chi, Hang
contents Magnetic topological insulators and their heterostructures provide great opportunities in coupling band topology with nontrivial spin configuration for enhanced spintronic device performance as well as designing totally new magnetoelectric systems and functionalities. We find that Mn interdiffusion from MnTe when interfaced with (Bi,Sb)2Te3 stabilizes as self-organized Mn(Bi,Sb)2Te4 septuple lamellae amongst alternating (Bi,Sb)2Te3 quintuple layers, as observed using scanning transmission electron microscopy and depth-sensitive polarized neutron reflectometry. We further demonstrate a valuable combination of magnetic and topological orders in these naturally formed Mn(Bi,Sb)2Te4-(Bi,Sb)2Te3 heterostructures that are exchange coupled with MnTe. Magnetotransport experiments and quantum magnetism simulations reveal that, above its own Neel temperature TN of 20 K, Mn(Bi,Sb)2Te4 mediates the exchange field leading to an anomalous Hall effect at the (Bi,Sb)2Te3/MnTe interface, with an enhanced interfacial TN exceeding 200 K. This novel magnetic interface in turn allows a robust and deterministic spin-orbit torque switching without an external magnetic field at a low critical current density of 300 kA cm-2. The antiferromagnetically coupled architecture of Mn(Bi,Sb)2Te4-(Bi,Sb)2Te3/MnTe, featuring unique magnetic and topological proximity effects across a chalcogenide backbone, is rich in fundamental interface physics and holds potential for practical applications in spintronics.
format Preprint
id arxiv_https___arxiv_org_abs_2604_18935
institution arXiv
publishDate 2026
record_format arxiv
spellingShingle Proximity Magnetism in Mn(Bi,Sb)2Te4-(Bi,Sb)2Te3/MnTe Natural Heterostructures
Vail, Owen A.
Wang, Shu-Wei
Hou, Yasen
Hettiarachchi, Dinura
Milette, Jean-Felix
Eldred, Tim B.
Gao, Wenpei
Sarney, Wendy
Ambaye, Haile
Keum, Jong
Lauter, Valeria
de Coster, George J.
Gilbert, Matthew J.
Heiman, Don
Moodera, Jagadeesh S.
Chi, Hang
Materials Science
Strongly Correlated Electrons
Magnetic topological insulators and their heterostructures provide great opportunities in coupling band topology with nontrivial spin configuration for enhanced spintronic device performance as well as designing totally new magnetoelectric systems and functionalities. We find that Mn interdiffusion from MnTe when interfaced with (Bi,Sb)2Te3 stabilizes as self-organized Mn(Bi,Sb)2Te4 septuple lamellae amongst alternating (Bi,Sb)2Te3 quintuple layers, as observed using scanning transmission electron microscopy and depth-sensitive polarized neutron reflectometry. We further demonstrate a valuable combination of magnetic and topological orders in these naturally formed Mn(Bi,Sb)2Te4-(Bi,Sb)2Te3 heterostructures that are exchange coupled with MnTe. Magnetotransport experiments and quantum magnetism simulations reveal that, above its own Neel temperature TN of 20 K, Mn(Bi,Sb)2Te4 mediates the exchange field leading to an anomalous Hall effect at the (Bi,Sb)2Te3/MnTe interface, with an enhanced interfacial TN exceeding 200 K. This novel magnetic interface in turn allows a robust and deterministic spin-orbit torque switching without an external magnetic field at a low critical current density of 300 kA cm-2. The antiferromagnetically coupled architecture of Mn(Bi,Sb)2Te4-(Bi,Sb)2Te3/MnTe, featuring unique magnetic and topological proximity effects across a chalcogenide backbone, is rich in fundamental interface physics and holds potential for practical applications in spintronics.
title Proximity Magnetism in Mn(Bi,Sb)2Te4-(Bi,Sb)2Te3/MnTe Natural Heterostructures
topic Materials Science
Strongly Correlated Electrons
url https://arxiv.org/abs/2604.18935